Pressure-induced quantum critical behavior and magnetic order in YbNi<sub>3</sub>Ga<sub>9</sub> with a chiral crystal structure: AC-calorimetric measurements up to 12 GPa

ORAL

Abstract

YbNi3X9 (X=Al, Ga) crystallize in the trigonal ErNi3Al9-type structure with a chiral space group R32. YbNi3Al9 undergoes a magnetic transition at TM=3.4 K. By substituting Cu for Ni, a chiral soliton lattice (CSL) is realized under magnetic fields B⊥c. While YbNi3Ga9 resides in an intermediate-valence regime under ambient pressure, application of pressure P is expected to drive this compound into a magnetic ordered state. Indeed, a magnetic order above Pc=9 GPa was inferred from the electrical resistivity and AC magnetic susceptibility measurements.
In this work, we have investigated the magnetic order in YbNi3Ga9 using AC-calorimetric measurements under P up to 12 GPa. With applying P, the Sommerfeld coefficient dramatically increases and reaches to 1 J/K2mol at 8.6 GPa≈Pc. A broad maximum in C/T at 1.6 K for P=9.3 GPa>Pc shifts to higher temperatures and becomes a sharp λ-type peak at 5 K for P≥11 GPa. The sets of data of C(T, P) under B//c and Bc at P≧11 GPa revealed that another field-induced ordered phase (FIOP) appears only for B⊥c. We discuss the origin of the FIOP in relation to the CSL for Yb(Ni1−xCux)3Al9 and A-phase for MnSi and EuPtSi.

*This work was partly supported by JSPS KAKENHI Grants No. JP16H01073 and No. JP18H04324, and JSPS Core-to-Core Program.

Presenters

  • Kazunori Umeo

    • N-BARD, Hiroshima University

Authors

  • Kazunori Umeo

    • N-BARD, Hiroshima University
  • Takumi Otaki

    • AdSM, Hiroshima University
  • Yudai Arai

    • AdSM, Hiroshima University
  • Shigeo Ohara

    • Graduate School of Engineering, Nagoya Institute of Technology
  • Toshiro Takabatake

    • Department of Quantum Matter, Hiroshima University
    • Hiroshima University
    • AdSM, Hiroshima University