Effect of Remote Surface Optical Phonon Scattering in Ferroelectric-Gated Single- and Bi-layer Graphene

ORAL

Abstract

We investigate the effect of the remote surface optical (RSO) phonon scattering on the transport properties of single and bi-layer graphene gated by ferroelectric Ba0.6Sr0.4TiO3 (BSTO) thin films. Graphene flakes were exfoliated on epitaxial 100-300 nm BSTO thin films grown on Nb-doped SrTiO3 substrates. Single and bi-layer samples were then identified via optical microscopy and characterized by atomic force microscopy and Raman spectra. Selected flakes were fabricated into field effect transistor (FET) devices via e-beam lithography. At low temperature, these ferroelectric-gated FETs (FeFET) exhibit resistivity hysteresis induced by ferroelectric switching, which evolves to anti-hysteresis at ~40 K. The graphene FETs exhibit high field effect mobility up to µFE~19,000 cm2/Vs and quantum Hall at 10 K, from which we deduced a dielectric constant of ~60 for BSTO. We examined the temperature dependence of the resistivity, which reveals dominant RSO phonon scattering from the interface with BSTO. We also discuss the effect of capping these samples with a top h-BN layer. Our study facilities the development of high-performance FeFETs based on graphene.

*This work was primarily supported by the U.S. Department of Energy, BES, under Award No. DE-SC0016153.

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Presenters

  • Hanying Chen

    • Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska - Lincoln
    • Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska-Lincoln

Authors

  • Hanying Chen

    • Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska - Lincoln
    • Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska-Lincoln

  • Zhiyong Xiao

    • Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska - Lincoln
    • Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska-Lincoln

  • Anil K Rajapitamahuni

    • Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska-Lincoln

  • Yifei Hao

    • Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska-Lincoln

  • Kenji Watanabe

    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305 0044, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science, , 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Material Science, 1-1 Namiki, Tsukuba 305-0044
    • National Institute of Materials Science
    • NIMS, Japan
    • Advanced Materials Laboratory, NIMS
    • National Institute for Materials Science, Tsukuba, Japan
    • National Institute for Materials Science, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Materials Science, 1-2-1 Sengen, Tsukuba, Ibaraki 305-0044, Japan
    • National Institute for Materials Science (NIMS)
    • NIMS Tsukuba
    • National Institute for Materials Science (Japan)
    • NIMS
    • National Institute for Material Science
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, Japan
    • National Institute for Materials Science , Japan
    • National Institute for Materials Science, Namiki 1-1, Tsukuba, Ibaraki 305-0044, Japan.
    • Advanced Materials Laboratory, National Institute for Materials Science, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan
    • National Institute for Materials Science, Tsukuba, Ibaraki 305- 0044, Japan
    • National Institute for Material Science - Japan
    • National Institute for Materials Science, Namiki Tsukuba Ibaraki, Japan
    • National Institute of Material Science
    • Advanced Material Lab, NIMS
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Ibaraki, Japan
    • National Institute for Materials Science, Tsukuba
    • 1-1 Namiki, Tsukuba, National Institute for Materials Science
    • NIMS/Tsukuba
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044 Japan
    • National Institute for Materials Science, Namiki, 305-0044, Japan
    • National Institute for Material Science, Japan
    • Advanced Materials Laboratory, NIMS, Japan
    • Columbia University
    • Advanced Materials Labaratory, National Institute for Materials Science
    • National Institute of Material Science, 1-1 Namiki, Tsukuba, Ibaraki 205-0044, Japan
    • National Institute of Materials Science, Japan

  • Takashi Taniguchi

    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305 0044, Japan
    • National Institute for Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science, , 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Material Science, 1-1 Namiki, Tsukuba 305-0044
    • National Institute of Materials Science
    • NIMS, Japan
    • Advanced Materials Laboratory, NIMS
    • National Institute for Materials Science, Tsukuba, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Materials Science, 1-2-1 Sengen, Tsukuba, Ibaraki 305-0044, Japan
    • National Institute for Materials Science (NIMS)
    • NIMS Tsukuba
    • NIMS
    • National Institute for Material Science
    • National Institute for Materials Science, Japan
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, Japan
    • National Institute for Materials Science , Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan
    • National Institute for Materials Science, Tsukuba, Ibaraki 305- 0044, Japan
    • National Institute for Material Science - Japan
    • National Institute for Materials Science, Namiki Tsukuba Ibaraki, Japan
    • National Institute of Material Science
    • Advanced Material Lab, NIMS
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Ibaraki, Japan
    • National Institute for Materials Science, Tsukuba
    • 1-1 Namiki, Tsukuba, National Institute for Materials Science
    • NIMS/Tsukuba
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044 Japan
    • National Institute for Materials Science, Namiki, 305-0044, Japan
    • National Institute for Material Science, Japan
    • Advanced Materials Laboratory, NIMS, Japan
    • Advanced Materials Labaratory, National Institute for Materials Science
    • National Institute of Material Science, 1-1 Namiki, Tsukuba, Ibaraki 205-0044, Japan
    • National Institute of Materials Science, Japan

  • Xia Hong

    • Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska - Lincoln
    • Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience, University of Nebraska-Lincoln
    • Univ of Nebraska - Lincoln