Perfectly gate-tunable graphene-WSe<sub>2</sub> van der Waal’s heterostructure at the Schottky-Mott limit

ORAL

Abstract

Recently, the Schottky-Mott (SM) limit has been studied through measurements on many metal-semiconductor junctions with various metals [1]. Here, we probe the SM limit using a single, gate-tunable, hexagonal boron nitride encapsulated graphene-WSe2-graphene heterostructure. One-dimensional edge contacts are made to the graphene and buried split-gates are used to separately tune the electrical properties each graphene-WSe2 junction. By making one graphene-WSe2 junction Ohmic, we perform electrical measurements of the Schottky barrier (SB) formed in the other junction. Electrical measurements of the SB show striking agreement with the ideal-diode equation, with over thirteen decades of drain current modulation via the gate voltage. Arrhenius activation energy measurements reveal one-to-one electrical control of the SB height by the gate voltage. These measurements indicate a stark absence of Fermi-level pinning at the graphene-WSe2 interface, resulting in a tunable SM limited heterojunction. Our findings are of broad significance, enabling fundamental studies of the SM limit and the ability to make superior electrical contact to two-dimensional materials.

[1] Y. Liu, J. Guo, E. Zhu, L. Liao, S.-J. Lee, M. Ding, I. Shakir, V. Gambin, Y. Huang, and X. Duan, Nature 557, 696 (2018).

Presenters

  • Samuel LaGasse

    • Colleges of Nanoscale Science and Engineering, SUNY Polytechnic Institute
    • Colleges of Nanoscale Science and Engineering, State University of New York Polytechnic Institute

Authors

  • Samuel LaGasse

    • Colleges of Nanoscale Science and Engineering, SUNY Polytechnic Institute
    • Colleges of Nanoscale Science and Engineering, State University of New York Polytechnic Institute
  • Prathamesh Dhakras

    • Colleges of Nanoscale Science and Engineering, SUNY Polytechnic Institute
    • SUNY Polytechnic Institute
    • Colleges of Nanoscale Science and Engineering, State University of New York Polytechnic Institute
  • Takashi Taniguchi

    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305 0044, Japan
    • National Institute for Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science, , 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Material Science, 1-1 Namiki, Tsukuba 305-0044
    • National Institute of Materials Science
    • NIMS, Japan
    • Advanced Materials Laboratory, NIMS
    • National Institute for Materials Science, Tsukuba, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Materials Science, 1-2-1 Sengen, Tsukuba, Ibaraki 305-0044, Japan
    • National Institute for Materials Science (NIMS)
    • NIMS Tsukuba
    • NIMS
    • National Institute for Material Science
    • National Institute for Materials Science, Japan
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, Japan
    • National Institute for Materials Science , Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan
    • National Institute for Materials Science, Tsukuba, Ibaraki 305- 0044, Japan
    • National Institute for Material Science - Japan
    • National Institute for Materials Science, Namiki Tsukuba Ibaraki, Japan
    • National Institute of Material Science
    • Advanced Material Lab, NIMS
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Ibaraki, Japan
    • National Institute for Materials Science, Tsukuba
    • 1-1 Namiki, Tsukuba, National Institute for Materials Science
    • NIMS/Tsukuba
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044 Japan
    • National Institute for Materials Science, Namiki, 305-0044, Japan
    • National Institute for Material Science, Japan
    • Advanced Materials Laboratory, NIMS, Japan
    • Advanced Materials Labaratory, National Institute for Materials Science
    • National Institute of Material Science, 1-1 Namiki, Tsukuba, Ibaraki 205-0044, Japan
    • National Institute of Materials Science, Japan
  • Kenji Watanabe

    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305 0044, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Materials Science
    • Advanced Materials Laboratory, National Institute for Materials Science, , 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Material Science, 1-1 Namiki, Tsukuba 305-0044
    • National Institute of Materials Science
    • NIMS, Japan
    • Advanced Materials Laboratory, NIMS
    • National Institute for Materials Science, Tsukuba, Japan
    • National Institute for Materials Science, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
    • National Institute for Materials Science, 1-2-1 Sengen, Tsukuba, Ibaraki 305-0044, Japan
    • National Institute for Materials Science (NIMS)
    • NIMS Tsukuba
    • National Institute for Materials Science (Japan)
    • NIMS
    • National Institute for Material Science
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, Japan
    • National Institute for Materials Science , Japan
    • National Institute for Materials Science, Namiki 1-1, Tsukuba, Ibaraki 305-0044, Japan.
    • Advanced Materials Laboratory, National Institute for Materials Science, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Ibaraki 305-0044, Japan
    • National Institute for Materials Science, Tsukuba, Ibaraki 305- 0044, Japan
    • National Institute for Material Science - Japan
    • National Institute for Materials Science, Namiki Tsukuba Ibaraki, Japan
    • National Institute of Material Science
    • Advanced Material Lab, NIMS
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Japan
    • Advanced Materials Laboratory, National Institute for Materials Science, Tsukuba, Ibaraki, Japan
    • National Institute for Materials Science, Tsukuba
    • 1-1 Namiki, Tsukuba, National Institute for Materials Science
    • NIMS/Tsukuba
    • National Institute for Materials Science, 1-1 Namiki, Tsukuba, 305-0044 Japan
    • National Institute for Materials Science, Namiki, 305-0044, Japan
    • National Institute for Material Science, Japan
    • Advanced Materials Laboratory, NIMS, Japan
    • Columbia University
    • Advanced Materials Labaratory, National Institute for Materials Science
    • National Institute of Material Science, 1-1 Namiki, Tsukuba, Ibaraki 205-0044, Japan
    • National Institute of Materials Science, Japan
  • Ji Ung Lee

    • Colleges of Nanoscale Science and Engineering, SUNY Polytechnic Institute
    • SUNY Polytechnic Institute
    • Colleges of Nanoscale Science and Engineering, State University of New York Polytechnic Institute