Capturing Dynamics of Incommensurate Antiferromagnetic Domains with Coherent Soft X-ray Scattering

ORAL

Abstract

The observation of antiferromagnetic (AFM) domains and the dynamics of their interfaces remains an elusive problem. The physical origin and dynamics of AFM domains are different from ferromagnetic domains and are largely unexplored. In this work, we have studied the frustrated AFM, Lu2CoMnO6, with the brilliant, coherent, soft X-ray flux of the 23ID-1 beamline at NSLS-II [1]. Lu2CoMnO6 is a double perovskite with frustrated AFM order leading to incommensurate ordering and dynamic time scales ranging from seconds to days [2-4]. We have probed the AFM domain structure and dynamics of this material with X-ray photon correlation spectroscopy (XPCS). The motion of the domains is revealed by the motion of a speckle pattern in the scattered X-ray beam. We observed faster domain fluctuations below onset of hysteresis at (35K) and explained these observations within the Axial Next-Nearest-Neighbor Ising (ANNNI) model.

References
[1] X. M. Chen, et al, Phys. Rev. Lett. 117, 167001 (2016).
[2] S. Yáñez-Vilar et al, Phys. Rev. B 84, 134427 (2011).
[3] S. Chikara et al, Phys. Rev. B 93, 180405(R) (2016).
[4] Vivien S. Zapf, et al, Phys. Rev. B 93, 134431 (2016).

Presenters

  • John Bowlan

    • Physical Chemistry and Applied Spectroscopy, Los Alamos National Laboratory

Authors

  • John Bowlan

    • Physical Chemistry and Applied Spectroscopy, Los Alamos National Laboratory
  • Richard L Sandberg

    • Center for Integrated Nanotechnologies, Los Alamos National Laboratory
    • Los Alamos National Laboratory
  • Vivien Zapf

    • National High Magnetic Field Laboratory, Los Alamos National Laboratory
    • Los Alamos National Laboratory
  • Xiaxin Ding

    • Idaho National Laboratory
    • National High Magnetic Field Laboratory, Los Alamos National Laboratory
    • Los Alamos National Laboratory
  • Shizeng Lin

    • Los Alamos National Laboratory
    • Theoretical Division, Los Alamos National Laboratory
  • Colby Walker

    • Center for Integrated Nanotechnologies, Los Alamos National Laboratory
  • Benjamin A Pound

    • Center for Integrated Nanotechnologies, Los Alamos National Laboratory
  • Nara Lee

    • Yonsei University
    • Yonsei Univ
  • Young Jai Choi

    • Yonsei University
    • Yonsei Univ
  • Andi Barbour

    • Brookhaven National Laboratory
    • NSLS-II, Brookhaven National Laboratory
    • BNL
  • Wen Hu

    • NSLS-II, Brookhaven National Laboratory
    • Brookhaven National Laboratory
  • Stuart B Wilkins

    • Brookhaven National Laboratory
    • NSLS-II, Brookhaven National Laboratory
    • National Synchrotron Light Source II, Brookhaven National Laboratory
    • BNL
  • Claudio Mazzoli

    • Brookhaven National Laboratory
    • NSLS-II, Brookhaven National Laboratory
    • National Synchrotron Light Source II, Brookhaven National Laboratory
    • BNL
    • Brookhaven National Lab