Transient superconductivity without superconductivity

ORAL

Abstract

Recent experiments on K3C60 and layered copper-oxide materials have reported substantial changes in the optical response following application of an intense THz pulse. These data have been interpreted as the stimulation of a transient superconducting state even at temperatures well above the equilibrium transition temperature. We propose an alternative phenomenology based on the assumption that the pulse creates a non-superconducting, though non-equilibrium situation in which the linear response conductivity is negative. The negative conductivity implies that the spatially uniform pre-pulse state is unstable and evolves to a new state with a spontaneous electric polarization. This state exhibits coupled oscillations of entropy and electric charge whose coupling to incident probe radiation modifes the reflectivity, leading to an apparently superconducting-like response that resembles the data. Dependencies of the reflectivity on polarization and angle of incidence of the probe are predicted and other experimental consequences are discussed.

*Basic Energy Sciences Division of the U.S. DOE grant DE-SC0018218
Simons Foundation

Presenters

  • Giuliano Chiriaco

    • Columbia University

Authors

  • Giuliano Chiriaco

    • Columbia University
  • Andrew Millis

    • Center for Computational Quantum Physics, Flatiron Institute
    • Physics, Columbia University
    • Columbia University
    • Department of Physics, Columbia University
    • Center for Computational Quantum Physics, Flatiron Institute, NY, NY, 10010
    • National Institute of Materials Science
    • Center for Computational Quantum Physics, Flatiorn Institute, Physics Department, Columbia University
  • Igor L Aleiner

    • Columbia University