Observation of the Charge-Stripe Crystal Phase in an Insulating Cuprate

ORAL

Abstract

High-temperature superconductivity in cuprates arises from carrier doping an antiferromagnetic Mott (AFM) insulator. This carrier doping leads to the formation of electronic liquid crystal phases. The insulating charge-stripe crystal phase is predicted to form when a small density of holes is doped into the charge-transfer insulator state, but this phase is yet to be experimentally observed. We realized the lightly-doped charge transfer insulating state of the cuprate Bi2Sr2CaCu2O8+x by surface annealing. In this insulating state with a charge transfer gap at the order of ~1 eV, we discovered a unidirectional charge-stripe order with a commensurate 4a0 period along the Cu-O-Cu bond. Notably, this insulating charge stripe crystal phase develops before the onset of the pseudogap and the formation of the Fermi surface. Our work provides fresh insight into the microscopic origin of electronic inhomogeneity in high-Tc cuprates.

*We gratefully acknowledge the support from the DARPA Grant NO. N66001-17-1-4051, Army Research Office Grant No. W911NF-17-1-0399 and the NSF Grant No. 1654041.

Presenters

  • He Zhao

    • Boston College

Authors

  • He Zhao

    • Boston College
  • Zheng Ren

    • Boston College
  • Bryan Rachmilowitz

    • Boston College
  • John A. Schneeloch

    • Brookhaven National Laboratory
    • Condensed Matter Physics & Materials Science, Brookhaven National Laboratory
    • Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory
    • University of Virginia
  • Ruidan Zhong

    • Brookhaven National Lab
    • Department of Chemistry, Princeton University
    • Department of Condensed Matter Physics and Materials Science, Brookhaven, Brookhaven National Laboratory, Upton, New York 11973-5000, USA.
    • Brookhaven National Laboratory
    • Condensed Matter Physics & Materials Science, Brookhaven National Laboratory
    • Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory
    • Brookhaven National Laboratories
  • Genda Gu

    • Brookhaven National Laboratory
    • Brookhaven National Lab
    • Department of Condensed Matter Physics and Materials Science, Brookhaven, Brookhaven National Laboratory, Upton, New York 11973-5000, USA.
    • Cond. Matt. Physics and Material Science, Brookhaven Natl Lab
    • Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory
    • Condensed Matter Physics & Materials Science Department, Brookhaven National Laboratory
    • Brookhaven National Labs, Long Island, NY, USA, 11973
    • Condensed Matter Physics & Materials Science, Brookhaven National Laboratory
    • Condensed Matter Physics, Brookhaven National Laboratory
    • Brookhaven National Laboratories
    • Chinese Academy of Sciences
    • Condensed Matter Physics & Materials Science, Brookhaven National Lab
    • Brookhaven Natl Lab
  • Ziqiang Wang

    • Department of Physics, Boston College
    • Boston College
    • Physics, Boston College
  • Ilija Zeljkovic

    • Boston College