Phase diagram of compressed RbEuFe<sub>4</sub>As<sub>4</sub> and CsEuFe<sub>4</sub>As<sub>4</sub>: Coexistence of superconductivity and magnetism

ORAL

Abstract

RbEuFe4As4 and CsEuFe4As4 are members of the recently discovered 1144 superconducting family, they exhibit the unusual combination of superconductivity (Tc ~ 35 K) and ferromagnetism (Tm ~ 15 K). We performed a series of measurements under compression including x-ray diffraction, magnetic susceptibility, and electrical resistivity. Compression monotonically suppresses Tc and enhances Tm. Near 7 GPa, Tc onset and Tm become comparable, at higher compression evidence of bulk superconductivity gradually disappears. Room-temperature x-ray diffraction measurements provide evidence of a transition from tetragonal to a half-collapse-tetragonal structure near 10 GPa for RbEuFe4As4 and near 12 GPa for CsEuFe4A4. The cross-over from ferromagnetic superconductor (Tc > Tm), to superconducting ferromagnet (Tm > Tc) occurs before the structural transition, suggesting that RbEuFe4As4 and CsEuFe4As4 are an ideal system for studying the interplay between superconductivity and magnetism.

*Equipment development partially supported by the NHMFL User Collaboration Grants Program, NSF Cooperative Agreement DMR-1157490 and the State of Florida, as well as DOE-NNSA DE-NA0002928. Measurements supported by NSF DMR-1453752, NSF EAR-1606856, and DFG MA 7362/1-1. DEJ aknowledges support from LDRD XWR500.

Presenters

  • Daniel Jackson

    • Pulsed Field Facility, National High Magnetic Field Laboratory, Los Alamos National Lab

Authors

  • Daniel Jackson

    • Pulsed Field Facility, National High Magnetic Field Laboratory, Los Alamos National Lab
  • Derrick VanGennep

    • Department of Physics, University of Florida
    • University of Florida
  • Wenli Bi

    • APS, Argonne National Lab
    • Advanced Photon Source, Argonne National Laboratory
    • Advanced Photon Source, Argonne National Laboratory, Argonne
  • Dongzhou Zhang

    • Hawaii Institute of Geophysics and Planetology, University of Hawaii at Manoa
  • Philipp Materne

    • Advanced Photon Source, Argonne National Laboratory
  • Yi Liu

    • Zhejiang University
    • Department of Physics, Zhejian University
  • Guang-Han Cao

    • Zhejiang University
    • Department of Physics, Zhejian University
  • Samuel T Weir

    • Physics Division, Lawrence Livermore National Laboratory
    • Lawrence Livermore Natl Lab
  • Yogesh Kumar Vohra

    • Department of Physics, University of Alabama at Birmingham
    • University of Alabama at Birmingham
  • James Hamlin

    • University of Florida
    • Department of Physics, University of Florida