Meeting a strange metal in heterostructures and thin films of LaNiO<sub>3</sub>

 · Invited

Abstract

The transition metal oxides are host to several ‘strange’ metals whose properties cannot be described within the paradigm of conventional Fermi liquids. Heterostructures incorporating such metals also have properties that are distinct from those found in similar structures using conventional metals. In this talk, I will present our work on epitaxial thin films of LaNiO3, and superlattices of La2/3Sr1/3MnO3/LaNiO3 grown using ozone-assisted molecular beam epitaxy. LaNiO3 is widely believed to be a paramagnetic metal down to the lowest temperatures, the only exception amongst the ReNiO3 rare earth nickelates. I will describe new insights from transport measurements in LaNiO3 about the nature of this strange metal. In addition, when LaNiO3 is placed in proximity with La2/3Sr1/3MnO3, interfacial charge transfer and exchange interactions give rise to striking phenomena, including a non-collinear helical magnetic structure in LaNiO3. These findings will be situated in the context of our current understanding of LaNiO3.

*The work was primarily funded by the Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division. The use of facilities at the Center for Nanoscale Materials, an Office of Science user facility, was supported by the US Department of Energy, Basic Energy Sciences under Contract No. DE-AC02-06CH11357. Work at Brookhaven National Laboratory is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. We acknowledge the support of the National Institute of Standards and Technology, U.S. Department of Commerce, in providing the neutron research facilities used in this work. The synchrotron based resonant x-ray scattering measurements were carried out at the Canadian Light Source, Saskatchewan, Canada, and SOLEIL, France.

Presenters

  • Anand Bhattacharya

    • Argonne National Laboratory
    • Materials Science Division, Argonne National Laboratory

Authors

  • Anand Bhattacharya

    • Argonne National Laboratory
    • Materials Science Division, Argonne National Laboratory