Superconductivity in Undoped CaFe<sub>2</sub>As<sub>2</sub> Single Crystals at Ambient Pressure

ORAL

Abstract

Among the many theoretical mechanisms proposed for higher Tc, the interfacial mechanism provides not only continual inspiration but also hope. For pristine CaAs2Fe2 (Ca122) single crystals, previous studies have shown the existence of complex phase, but no superconductivity was reported at ambient pressure. Recently, we identified two different non-superconducting phases in Ca122 through thermal treatments. Such thermal treatments offer a reproducible, controllable, and reversible environment in which many characterization techniques can be applied. We successfully tuned a mixed-phase in Ca122 through a proper annealing process and induced the superconductivity with a Tc up to 25 K at ambient pressure[1]. The transport, magnetic, and room temperature X-ray results lead us to the conjecture that the origin of superconductivity arises from the interface of the mesoscopically stacked layers of PI and PII. To further understand the underlying mechanism, systematic low-temperature X-ray, STEM, and high-pressure measurements were conducted over a series of thermal treated Ca122 single crystals[2]. This work provides the first direct evidence of interfacial induced superconductivity in undoped Ca122 single crystals.

Presenters

  • Liangzi Deng

    • Texas Center for Superconductivity
    • Department of Physics and Texas Center for Superconductivity, University of Houston
    • Department of Physics and Texas Center for Superconductivity at University of Houston

Authors

  • Liangzi Deng

    • Texas Center for Superconductivity
    • Department of Physics and Texas Center for Superconductivity, University of Houston
    • Department of Physics and Texas Center for Superconductivity at University of Houston
  • Shuyuan Huyan

    • Texas Center for Superconductivity
    • Department of Physics and Texas Center for Superconductivity, University of Houston
    • Department of Physics and the Texas Center for Superconductivity, University of Houston
    • Department of Physics and Texas Center for Superconductivity at University of Houston
  • Kui Zhao

    • Texas Center for Superconductivity
    • Department of Physics and Texas Center for Superconductivity, University of Houston
  • Wu Zheng

    • Texas Center for Superconductivity
  • Bing Lv

    • University of Texas at Dallas
    • Department of Physics, University of Texas at Dallas
    • Univ of Texas, Dallas
    • Dept. of Physics, The University of Texas at Dallas
    • Department of Physcis, University of Texas at Dallas
  • Jingying Sun

    • Texas Center for Superconductivity
    • Department of Physics and Texas Center for Superconductivity, University of Houston
    • Department of Physics and the Texas Center for Superconductivity, University of Houston
    • Department of Physics and Texas Center for Superconductivity at University of Houston
  • Shuo Chen

    • Department of Physics and TcSUH, University of Houston
    • Texas Center for Superconductivity
    • Department of Physics and Texas Center for Superconductivity, University of Houston
    • Department of Physics and the Texas Center for Superconductivity, University of Houston
    • Department of Physics and Texas Center for Superconductivity at University of Houston
    • Univ of Houston
  • Lijun Wu

    • Condensed Matter Physcis and Materials Science Departement, Brookhaven National Laboratory
    • Brookhaven National Laboratory
    • Brookhaven Natl Lab
  • Yimei Zhu

    • Condensed Matter Physcis and Materials Science Departement, Brookhaven National Laboratory
    • Brookhaven National Laboratory
    • Condensed Matter Physics & Materials Science, Brookhaven National Laboratory
    • Brookhaven Natl Lab
    • Brookhaven National Lab
    • Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory
    • Department of Condensed Matter Physics and Materials Science, Brookhaven National Laboratory
    • Condensed Matter Physics & Materials Science Department, Brookhaven National Laboratory
  • Melissa Gooch

    • Texas Center for Superconductivity
    • Department of Physics and Texas Center for Superconductivity, University of Houston
    • Texas Center for Superconductivity at the University of Houston
  • Paul Chu

    • Texas Center for Superconductivity
    • Department of Physics and Texas Center for Superconductivity, University of Houston
    • Department of Physics and the Texas Center for Superconductivity, University of Houston
    • Department of Physics and Texas Center for Superconductivity at University of Houston