Superionic Diffusion Through Frustrated Energy Landscape

ORAL

Abstract

Solid-state materials with extremely high ionic diffusion are necessary to many technologies including all-solid-state Li-ion batteries. Despite the strong efforts made towards the search for crystal structures leading high lithium diffusion, only a handful crystalline structure families have been reported as Li superionic conductors.
In this work, we demonstrate that LiTi2(PS4)3, or LTPS, shows exceptional Li-ion diffusion an order of magnitude higher than current state-of-the-art superionic conductors. By means of extensive theoretical studies through ab initio molecular dynamics (backed up by several experimental characterization), we rationalize the exceptional performances of this new superionic conductor through the concept of frustrated energy landscape. The absence of regular and undistorted sites for Li leads to low diffusion energy barrier as well as an exceptional pre-factor.
Our work not only sheds light on a new family of superionic conductors but offers a new design principle for discovering new ones.

Presenters

  • Davide Di Stefano

    • Université catholique de Louvain

Authors

  • Davide Di Stefano

    • Université catholique de Louvain
  • Anna Miglio

    • Institute of Condensed Matter and Nanoscience, ETSF, Université Catholique de Louvain
    • Université catholique de Louvain
  • Koen Robeyns

    • Université catholique de Louvain
  • Yaroslav Filinchuk

    • Université catholique de Louvain
  • Marine Lechartier

    • Toyota Motor Europe
  • Anatoliy Senyshyn

    • Heinz Maier-Leibnitz Center, Technical University Munich
    • Technische Universitaet Muenchen
    • Heinz Maier-Leibnitz Zentrum, Technische Universitat Munchen
  • Hiroyuki Ishida

    • Toray Research Center Inc.
  • Stefan Spannenberger

    • Philipps-Universitaet Marburg
  • Bernhard Roling

    • Philipps-Universitaet Marburg
  • Denise Prutsch

    • Graz University of Technology
  • Daniel Rettenwander

    • Graz University of Technology
  • Martin Wilkening

    • Graz University of Technology
  • Yuki Katoh

    • Toyota Motor Europe
  • Geoffroy Hautier

    • Institute of Condensed Matter and Nanosciences, Université Catholique de Louvain
    • Univ Catholique de Louvain
    • IMCN, Université Catholique de Louvain
    • Université catholique de Louvain