Phase Competition in the Palmer-Chalker XY Pyrochlore Er<sub>2</sub>Pt<sub>2</sub>O<sub>7</sub>

ORAL

Abstract

We report neutron scattering measurements on Er2Pt2O7, a new addition to the XY family of frustrated pyrochlore magnets. Symmetry analysis of our elastic scattering data shows that Er2Pt2O7 orders into the k = 0, Γ7 magnetic structure (the Palmer-Chalker state), at 0.38 K. This contrasts with its sister XY pyrochlore antiferromagnets Er2Ti2O7 and Er2Ge2O7, both of which order into Γ5 magnetic structures at much higher temperatures, 1.2 and 1.4 K, respectively. Below TN = 0.38 K, Er2Pt2O7 displays a gapped spin-wave spectrum with an intense, flat band of excitations at lower energy and a weak, diffusive band of excitations at higher energy. The flat band is well described by classical spin-wave calculations, but these calculations also predict sharp dispersive branches at higher energy, a striking discrepancy with the experimental data. This, in concert with the strong suppression of TN, is attributable to enhanced quantum fluctuations due to phase competition between the Γ7 and Γ5 states that border each other within a classically predicted phase diagram.

*The work was supported by the Natural Sciences and Engineering Research Council of Canada.

Presenters

  • Alannah Hallas

    • Physics and Astronomy, Rice University
    • McMaster Univ
    • Rice University

Authors

  • Alannah Hallas

    • Physics and Astronomy, Rice University
    • McMaster Univ
    • Rice University
  • Jonathan Gaudet

    • McMaster Univ
    • McMaster University
  • Nicholas Butch

    • NIST Center for Neutron Research, National Institute of Standards and Technology
    • NIST Center for Neutron Research
    • NIST- Natl Inst of Stds & Tech
    • Center for Neutron Research, NIST -Natl Inst of Stds & Tech
    • NIST -Natl Inst of Stds & Tech
    • NIST center for neutron research
    • NIST
  • Guangyong Xu

    • NCNR, National Institute of Standards and Technology
    • NIST Center for Neutron Research, National Institute of Standards and Technology
    • NIST -Natl Inst of Stds & Tech
    • NIST Center for Neutron Research
    • NIST
  • Makoto Tachibana

    • National Institute for Material Research
    • National Institute of Materials Science
    • NIMS
  • Christopher Wiebe

    • Chemistry, University of Winnipeg
    • University of Winnipeg
  • Graeme Luke

    • McMaster University
    • Physics and Astronomy, McMaster University
    • Department of Physics and Astronomy, McMaster Univ
    • Department of Physics and Astronomy, McMaster University
    • Physics and Astronomy, McMaster Univ
    • MacMaster University
    • Physics, McMaster University
    • McMaster Univ
  • Bruce Gaulin

    • Department of Physics and Astronomy, McMaster University
    • McMaster Univ
    • McMaster University