Imaging Synthetic Polymer Crystals and Defects on Atomic Length-Scales

ORAL

Abstract

Determining atomic-scale structures in polymers is difficult because they degrade rapidly when studied by electron microscopy, and techniques such as x-ray scattering average over volumes much larger than the unit cells. We obtained cryo-electron microscopy images of crystals of a peptoid polymer in which we see a variety of crystalline motifs. A combination of crystallographic and single particle methods, developed for cryo-electron microscopy of biological macromolecules, was used to obtain high resolution images of the crystals. Individual specimens contain grains that are mirror images of each other with concomitant grain boundaries. Our approach is robust and may enable direct visualization of crystalline grains and grain boundaries on atomic length scales in a variety of polymers.

*Funding for this work was provided by the Soft Matter Electron Microscopy Program (KC11BN), supported by the Office of Science, Office of Basic Energy Science, US Department of Energy, under Contract DE-AC02-05CH11231.

Presenters

  • Nitash Balsara

    • Univ of California - Berkeley
    • Chemical and Biomolecular Engineering, University of California, Berkeley
    • University of California Berkeley

Authors

  • Nitash Balsara

    • Univ of California - Berkeley
    • Chemical and Biomolecular Engineering, University of California, Berkeley
    • University of California Berkeley
  • Xi Jiang

    • Univ of California - Berkeley
  • Douglas Greer

    • Univ of California - Berkeley
  • Kenneth Downing

    • Univ of California - Berkeley
  • Ronald Zuckermann

    • Lawrence Berkeley National Laboratory
    • Molecular Foundry, Lawrence Berkeley National Laboratory
    • Univ of California - Berkeley
  • Joyjit Kundu

    • Duke Univ
    • Univ of California - Berkeley
  • David Prendergast

    • LBNL
    • Lawrence Berkeley National Laboratory
    • Lawrence Berkeley Natl Lab
    • Lawrence Berkeley National Lab
    • Univ of California - Berkeley