Terahertz spectroscopy of strongly frustrated helical magnet Fe<sub>3</sub>PO<sub>4</sub>O<sub>3</sub>

ORAL

Abstract

The hexagonal lattice in Fe3PO4O3 is made up of three triangularly coordinated Fe units that make the magnetic interactions strongly geometrically frustrated. Along the c-axis, layers of these triangular units arrange in a larger, triangular lattice pattern, making the magnetic interactions also frustrated. Even with this level of frustration, magnetic order occurs below TN ~ 165 K in the form of a long-wavelength helical pattern. We use time-domain terahertz (THz) spectroscopy to study the magnetic excitations in powder samples of this material. We find an overall softening of the magnetic spectrum around TN, but with no well-defined sharp resonant modes. However, below ~40 K we find a well defined resonant mode centered around ~ 900 GHz suggesting the existence of an additional transition below this temperature. We will discuss the possible explanations of this behavior within linear spin-wave theory.

*Patial support was provided by the Center for Emergent Materials, an NSF MRSEC, under grant DMR-1420451.

Presenters

  • Nicholas Crescimanno

    • Center for Emergent Materials. Department of Physics, The Ohio State University

Authors

  • Nicholas Crescimanno

    • Center for Emergent Materials. Department of Physics, The Ohio State University
  • Thuc Mai

    • Department of Physics, Ohio State Univ - Columbus
    • Physics, Ohio State University - Columbus
    • Center for Emergent Materials. Department of Physics, The Ohio State University
    • Department of Physics , The Ohio State University
  • Michael Tarne

    • Department of Chemistry , Colorado State University
  • Kate Ross

    • Physics, Colorado State University
    • Department of Physics, Colorado State University
    • Colorado State University
  • James Neilson

    • Chemistry, Colorado State University
    • Colorado State University
    • Department of Chemistry , Colorado State University
  • Rolando Valdes Aguilar

    • Department of Physics, Ohio State Univ - Columbus
    • Center for Emergent Materials. Department of Physics, The Ohio State University
    • Physics, Ohio State University - Columbus
    • Ohio State Univ - Columbus
    • Department of Physics , The Ohio State University