Field dependence of magnetic order and excitations in the Kitaev candidate alpha-RuCl3

ORAL

Abstract

The search for new quantum states of matter has been one of the forefront endeavors of condensed matter physics. ~The two-dimensional Kitaev quantum spin liquid (QSL) is of special interest as an exactly solvable spin-liquid model exhibiting exotic fractionalized excitations. Recently, alpha-RuCl3 has been identified as a candidate system for exhibiting some aspects of Kitaev QSL physics.~ ~The spins in this material exhibit zig-zag order at low temperatures, and show both low energy spin wave excitation arising from the ordered state as well as a continuum excitation extending to higher energies that has been taken as evidence for QSL relate Majorana fermions.~ ~In this talk, we show that the application of an in-plane magnetic field suppresses the zig-zag order possibly resulting in a state devoid of long-range order. Field-dependent inelastic neutron scattering on single-crystal shows a remarkable effect on the excitation spectrum above the critical field.

*The work is supported by US-DOE, Office of Science, Basic Energy Sciences and User Facilities Divisions, and also the Gordon and Betty Moore Foundation EPiQS grant GBFM4416.

Authors

  • Arnab Banerjee

    • Quantum Condensed Matter Division, Oak Ridge National Laboratory
  • Paula Kelley

    • Material Science and Technology Division, Oak Ridge National Laboratory
  • Barry Winn

    • Quantum Condensed Matter Division, Oak Ridge National Laboratory
  • A.A. Aczel

    • Quantum Condensed Matter Division, Oak Ridge National Laboratory
    • Oak Ridge National Lab
    • Oak Ridge National Laboratory
  • Mark Lumsden

    • Quantum Condensed Matter Division, Oak Ridge National Laboratory
    • ORNL
  • David Mandrus

    • Material Science and Technology Division, Oak Ridge National Laboratory
  • Stephen Nagler

    • Quantum Condensed Matter Division, Oak Ridge National Laboratory