First principles calculations of the two dimensional topological insulator stanene on substrates

ORAL

Abstract

Topological insulators are a class of materials under continued intense investigation due to their potentially robust current carrying surface or edge states. Stanene, the two dimensional form of tin, has been predicted to be a 2D topological insulator due to its large spin-orbit interaction. There exist a number of first principles calculations of stanene both as an isolated layer as well as on a substrate, but the only successful experimental report involves the growth of stanene on Bi$_2$Te$_3$, and does not show signatures of topological behavior.* In this work, we present first-principles density functional theory calculations of stanene on a Bi$_2$Te$_3$ substrate and report on the binding, interfacial structure, and role of various decorating groups ({\it i.e.}, atoms or molecules binding to stanene). In addition, we will describe the possible benefits of using wide gap insulators such as CdTe as substrates.\\ $^*$F. Zhu, W. Chen, Y. Xu, C. Gao, D. Guan, C. Liu, D. Qian, S.-C. Zhang, and J. Jia, {\it Nat.\ Mater.}\ (2015).

*This work is supported by Functional Accelerated nanoMaterial Engineering (FAME).

Authors

  • Stephen Eltinge

    • Department of Physics, Yale University
    • Yale University
  • Minjung Kim

    • Department of Applied Physics, Yale University
    • Yale University
  • Stephen Albright

    • Department of Physics, Yale University
    • Department of Physics and Center for Research on Interface Structures and Phenomena (CRISP), Yale University
    • Yale University
  • Rui Peng

    • Department of Applied Physics, Yale University
    • Department of Applied Physics and CRISP, Yale University
  • Ke Zou

    • Department of Applied Physics, Yale University
    • Department of Applied Physics and CRISP, Yale University
    • Dept. of Appl. Phys. and CRISP, Yale Univ.
    • Yale University
  • Frederick Walker

    • Department of Applied Physics, Yale University
    • Yale Univ
    • Department of Applied Physics and CRISP, Yale University
    • Yale University
  • Charles Ahn

    • Department of Applied Physics, Yale University
    • Yale Univ
    • Department of Applied Physics and CRISP, Yale University
    • Yale University
  • Sohrab Ismail-Beigi

    • Department of Applied Physics, Yale University
    • Center for Research on Interface Structures and Phenomena and Department of Applied Physics, Yale University
    • Yale Univ
    • Yale University