Absence of Superconductivity in Doping Kagome Quantum Spin Liquid

ORAL

Abstract

We study the effects of doping a Mott insulator on the kagome lattice where spins interact via antiferromagnetic Heisenberg couplings. This model is known to have a quantum spin liquid ground state at half-filling. The effect of hole doping is studied within the context of the t-J model using large-scale density-matrix renormalization group. Surprisingly, we find that there is no long-range superconductivity in the ground states of the system although the spin-spin correlations remain short-ranged for doping concentrations up to 11\%. The effective interaction between doped holes is repulsive. The ground states have robust long-range charge density wave order, which is either unidirectional stripe or two-dimensional Wigner crystal, whose pattern depends on the lattice geometry and hole doping concentration. These results may be relevant to kagome lattice Herbertsmithite ZnCu3(OH)6Cl2 upon doping.

Authors

  • Thomas Devereaux

    • Stanford Unviersity
    • Stanford Institute for Materials and Energy Sciences, Stanford University & SLAC
    • SLAC National Accelerator Laboratory
    • SLAC National Accelerator Laboratory, Stanford Institute for Materials and Energy Sciences
    • Geballe Laboratory for Advanced Materials, Stanford University, Stanford, CA, USA
    • Stanford Univ
    • SLAC National Accelerator Laboratory/Stanford University
    • Stanford Institute for Material and Energy Sciences
  • Hongchen Jiang

    • SLAC National Accelerator Laboratory
    • Stanford Institute for Materials and Energy Sciences, SLAC
    • Stanford Institute for Materials and Energy Sciences
  • Shenxiu Liu

    • Stanford Institute for Materials and Energy Sciences
  • Steve Kivelson

    • Stanford Univ