Giant Spin Gap and Magnon Localization in the Disordered Heisenberg Antiferromagnet Sr2Ir1-xRuxO4

ORAL

Abstract

We study the evolution of magnetic excitations in the disordered two-dimensional antiferromagnet Sr\textunderscore 2Ir\textunderscore 1-xRu\textunderscore xO\textunderscore 4. A gigantic magnetic gap greater than 40 meV opens at x $=$ 0.27 and increases with Ru concentration, from 40 meV to \textgreater 150 meV, rendering the dispersive magnetic excitations in Sr2IrO4 almost momentum independent. Up to a Ru concentration of x $=$ 0.77, both experiments and first-principles calculations show the Ir J\textunderscore eff $=$ 1/2 state remains intact. The magnetic gap arises from the local interaction anisotropy in the proximity of the Ru disorder. Under the coherent potential approximation, we reproduce the experimental magnetic excitations using the disordered Heisenberg antiferromagnetic model with suppressed next-nearest neighbor ferromagnetic coupling. Ref: Y. Cao et al., arXiv:1608.04640 (2016).

Authors

  • Yue Cao

    • Brookhaven National Laboratory
    • Brookhaven National Lab
    • Univ of Colorado - Boulder
  • Xuerong Liu

    • Institute of Physics, Chinese Academy of Sciences
  • Wenhu Xu

    • Brookhaven National Lab
  • Weiguo Yin

    • Brookhaven National Lab
  • Derek Meyers

    • Brookhaven National Lab
  • Jungho Kim

    • Advanced Photon Source, Argonne National Lab
  • Diego Casa

    • Advanced Photon Source, Argonne National Lab
  • Mary Upton

    • Advanced Photon Source, Argonne National Lab
  • Thomas Gog

    • Advanced Photon Source, Argonne National Lab
  • Tom Berlijn

    • Oak Ridge National Lab
  • Gonzalo Alvarez

    • Oak Ridge National Lab
  • Shujuan Yuan

    • Department of Physics and Astronomy, University of Kentucky
  • Jasminka Terzic

    • Department of Physics and Astronomy, University of Kentucky
  • J. M. Tranquada

    • Brookhaven National Lab
  • John Hill

    • Brookhaven National Lab
  • Gang Cao

    • Department of Physics, University of Colorado at Boulder
  • Robert Konik

    • Brookhaven National Lab
  • M. P. M. Dean

    • Brookhaven National Lab