New type of in-gap states at a spinel/perovskite interface: combined resonant soft x-ray photoemission spectroscopy and first-principles study.

ORAL

Abstract

Oxygen vacancies in oxide heterostructures create a plethora of electronic phenomena not observed in the stoichiometric systems. In this talk we will discuss the presence of a new type of in-gap states at the spinel/perovskite $\gamma$-Al$_2$O$_3$/SrTiO$_3$ interface [1,2], as observed in soft x-ray resonant photoemission spectroscopy. Based on \textit{ab initio} calculations and crystal-field analysis of different atomic environments, we identify the origin of this behavior and we argue on the possible origin of the extraordinarily high electron mobility measured in this heterostructure [2].\newline [1] P. Schuetz et al., in preparation.\newline [2] Y. Z. Chen et al., Nature Communications 4, 1371 (2013).

*This work was financially supported by the Deutsche Forschungsgemeinschaft SFB/TR 49 and SFB 1170.

Authors

  • Vladislav Borisov

    • Goethe University Frankfurt am Main, Germany
  • Philipp Schuetz

    • University of Wuerzburg, Germany
  • Florian Pfaff

    • University of Wuerzburg, Germany
  • Philipp Scheiderer

    • University of Wuerzburg, Germany
  • Lenart Dudy

    • University of Wuerzburg, Germany
  • Michael Zapf

    • University of Wuerzburg, Germany
  • Judith Gabel

    • University of Wuerzburg, Germany
  • Dennis Valbjorn Christensen

    • Technical University of Denmark
  • Yunzhong Chen

    • Technical University of Denmark
  • Nini Pryds

    • Technical University of Denmark
  • Vladimir Strocov

    • Swiss Light Source, Switzerland
  • Victor Rogalev

    • Swiss Light Source, Switzerland
  • Christoph Schlueter

    • Diamond Light Source, United Kingdom
  • Tien-Lin Lee

    • Diamond Light Source, United Kingdom
  • Harald O. Jeschke

    • Goethe University Frankfurt am Main, Germany
  • Roser Valenti

    • Goethe University Frankfurt am Main, Germany
  • Michael Sing

    • University of Wuerzburg, Germany
  • Ralph Claessen

    • University of Wuerzburg, Germany