Suppressed magnetism in Ca$_2$RuO$_4$ under applied electric currents

ORAL

Abstract

The $4d$-electron system Ca$_2$RuO$_4$ plays host to an exciting interplay between spin-orbit coupling and electronic correlation energies that gives rise to exotic ground states and a high sensitivity to external perturbation. Isovalent Sr-doping, hydrostatic pressure and even applied electric currents can induce dramatic changes in the exhibited electronic and magnetic properties. Here, we use single crystal neutron diffraction with in-situ applied electric currents to show that a previously identified current induced metal-insulator transition is linked to a modified distortion of the RuO$_6$ octahedra and a concomitant suppression of antiferromagnetic order. These results indicate a close correlation among the crystal lattice, electronic, and magnetic structures.

Authors

  • Joel Bertinshaw

    • Max Planck Institute for Solid State Research
  • Namrata Gurung

    • Max Planck Institute for Solid State Research
  • Maximilian Krautloher

    • Max Planck Institute for Solid State Research
  • Anil Jain

    • Max Planck Institute for Solid State Research
  • Juan Porras

    • Max Planck Institute for Solid State Research
  • Oscar Fabelo Rosa

    • Institut Laue-Langevin
  • BJ Kim

    • Max Planck Institute for Solid State Research
  • Bernhard Keimer

    • Max Planck Institute for Solid State Research