Hybrid magnon-phonons in the paraelectric antiferromagnet EuTiO$_{3}$

ORAL

Abstract

Magnetic perovskite titanate EuTiO$_{3}$ has attracted a lot of attentions for its large spin-lattice coupling. It has a number of similarities with the well-studied quantum paraelectric SrTiO$_{3}$ but a much higher cubic-tetragonal lattice transition at 290 K and an extra magnetic order at 5.5 K. The large difference between EuTiO$_{3}$ and SrTiO$_{3}$ has been attributed to the magnetic ion Eu$^{2+}$, that couples with the structural properties. However the spin-lattice coupling mechanism has not been fully understood yet although many theoretical models have been proposed. We grew a large, high-quality isotopically-enriched EuTiO$_{3}$ crystal for neutron scattering.~ The crystal and magnetic structures were calibrated with neutron diffraction at HB-3A at HFIR at ORNL at temperatures from 1.5 K to 450 K. The spin waves and phonons were measured in the temperature range of 1.5-400 K with HB-3 at HFIR, CNCS and ARCS at SNS at ORNL. I will report our new discovery of interaction between the soft ferroelectric phonon mode and likely (para)magnon mode, that is responsible for a giant magnetoelectric coupling in EuTiO$_{3}$. The magnetic excitation and atomic displacements will be discussed.

*This work was supported by Office of Basic Energy Sciences, U.S. Department of Energy.

Authors

  • Huibo Cao

    • Quantum Condensed Matter Division, Oak Ridge National Laboratory, Oak Ridge, TK 37831, USA
    • Oak Ridge National Laboratory
    • Quantum Condensed Matter Division, Oak Ridge National Laboratory
  • Olivier Delaire

    • Duke University
  • Jiawang Hong

    • Beijing Institute of Technology
  • Steven Hahn

    • Oak Ridge National Laboratory
  • Songxue Chi

    • Oak Ridge National Laboratory
  • George Ehlers

    • Oak Ridge National Laboratory
  • Douglas Abernathy

    • Oak Ridge National Laboratory
  • Andrew Christianson

    • Oak Ridge National Laboratory
  • Jaime Fernandez-Baca

    • Oak Ridge National Laboratory
  • Bryan Chakoumakos

    • Oak Ridge National Laboratory
  • Jiaqiang Yan

    • Oak Ridge National Laboratory
  • Brian Sales

    • Oak Ridge National Laboratory