Observation of interacting polaronic gas behavior in Ta-doped TiO$_{2}$ thin films via terahertz time-domain spectroscopy
ORAL
Abstract
Using terahertz time-domain spectroscopy (THz-TDS), we obtained the complex optical conductivity [$\tilde{\sigma} (\omega)$] of Ta-doped TiO$_{2}$ thin films --- a transparent conducting oxide (TCO), in the frequency range 0.3--2.7~THz, temperature range 10--300~K and various Ta dopings. Our results reveal the existence of an interacting polaronic gas in these TCOs, and suggest that their large conductivity is caused by the combined effects of large carrier density \textit{and} small electron-phonon coupling constant due to Ta doping.
*NUSNNI-NanoCore, NRF-CRP (NRF2008NRF-CRP002-024), NUS cross-faculty grant and FRC (ARF Grant No. R-144-000-278-112), MOE Tier 1 (RG123/14), SinBeRISE CREATE
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