Thermodynamic and electrical transport properties of the layered triangular Ce lattice compound CeAuAl4Ge2

ORAL

Abstract

We report electronic and magnetic properties of single crystalline CeAuAl$_{\mathrm{4}}$Ge$_{\mathrm{2}}$. This compound crystallizes in a rhombohedral structure (S.G. {\#}166) and may host geometrical magnetic frustration on the Ce sub-lattice. Electrical transport measurements show metallic behavior with a small residual resistivity ($\rho_{\mathrm{0}}$ $=$ 3 $\mu \Omega $cm). Quantum oscillations are seen in the ac magnetic susceptibility, which uncover a three-dimensional Fermi surface. Weak hybridization between the f- and conduction electron states is indicated by the simple-metallic temperature dependence of the electrical resistivity, the small electronic coefficient of the heat capacity, and the small charge carrier effective masses ($m$* $\approx $ 0.4 - 1 $m_{\mathrm{e}})$. As evidenced by the magnetic susceptibility, there is an appreciable difference between the Curie-Weiss temperature ($\Theta \quad \approx $ -90 K) and the onset of the magnetic ordering temperature ($T_{\mathrm{M}} \quad =$ 1.4 K), suggesting that magnetic frustration dominates the magnetic behavior. We will discuss the prospects for studying magnetic frustration in a simple metallic environment, and for tuning the magnetic ordering towards a frustrated quantum phase transition.

*This work was performed at the NHMFL, which is supported by NSF Cooperative Agreement No. DMR-0084173, the State of FL and the DOE. A portion of this work was supported by the NHMFL UCGP.

Authors

  • Shengzhi Zhang

    • National High Magnetic Field Lab,Tallahassee
  • Andrew Gallagher

    • Florida State University
    • National High Magnetic Field Lab,Tallahassee
  • You Lai

    • National High Magnetic Field Lab,Tallahassee
  • David Graf

    • National High Magnetic Field Laboratory
    • NHMFL
    • National High Magnetic Field Laboratory.
    • National High Magnetic Field Laboratory Tallahassee
    • Florida State University
    • National High Magnetic Field Lab,Tallahassee
  • Tiglet Besara

    • National High Magnetic Field Laboratory / Florida State University
    • National High Magnetic Field Laboratory: Florida State University
    • National High Magnetic Field Lab,Tallahassee
    • National High Magnetic Field Laboratory
  • Kuan-wen Chen

    • NHMFL and FSU
    • National High Magnetic Field Lab,Tallahassee
  • Theo Siegrist

    • National High Magnetic Field Laboratory / Florida State University
    • National High Magnetic Field Lab,Tallahassee
  • Laura Greene

    • 2017 APS President, National High Magnetic Field Laboratory, Florida State University
    • Florida State University
    • National High Magnetic Field Lab,Tallahassee
  • Ryan Baumbach

    • NHMFL
    • National High Magnetic Field Laboratory
    • Florida State University
    • National High Magnetic Field Lab,Tallahassee