High-Resolution Structural and Electronic Properties of Epitaxial Topological Crystalline Insulator Films

ORAL

Abstract

Revealing the local electronic properties of surfaces and their link to structural properties is an important problem for topological crystalline insulators (TCI) in which metallic surface states are protected by crystal symmetry. The microstructure and electronic properties of TCI SnTe film surfaces grown by molecular beam epitaxy were characterized using scanning probe microscopy. These results reveal the influence of various defects on the electronic properties: tilt boundaries leading to dislocation arrays that serve as periodic nucleation sites for pit growth; screw dislocations, and point defects. These features have varying length scale and display variations in the electronic structure of the surface, which are mapped with scanning tunneling microscopy images as standing waves superimposed on atomic scale images of the surface topography that consequently shape the wave patterns. Since the growth process results in symmetry breaking defects that patterns the topological states, we propose that the scanning probe tip can pattern the surface and electronic structure and enable the fabrication of topological devices on the SnTe surface.

*Financial support from the National Science Foundation through the Yale Materials Research Science and Engineering Center (Grant No. MRSEC DMR-1119826) and FAME.

Authors

  • Omur Dagdeviren

    • Yale Univ
    • Yale University
  • Chao Zhou

    • Yale Univ
    • Yale University
  • Ke Zou

    • Department of Applied Physics, Yale University
    • Department of Applied Physics and CRISP, Yale University
    • Dept. of Appl. Phys. and CRISP, Yale Univ.
    • Yale University
  • Georg Simon

    • Yale University
  • Stephen Albright

    • Department of Physics, Yale University
    • Department of Physics and Center for Research on Interface Structures and Phenomena (CRISP), Yale University
    • Yale University
  • Subhasish Mandal

    • Yale University
  • Mayra Morales-Acosta

    • Yale University
  • Xiaodong Zhu

    • Yale University
  • Sohrab Ismail-Beigi

    • Department of Applied Physics, Yale University
    • Center for Research on Interface Structures and Phenomena and Department of Applied Physics, Yale University
    • Yale Univ
    • Yale University
  • Frederick Walker

    • Department of Applied Physics, Yale University
    • Yale Univ
    • Department of Applied Physics and CRISP, Yale University
    • Yale University
  • Charles Ahn

    • Department of Applied Physics, Yale University
    • Yale Univ
    • Department of Applied Physics and CRISP, Yale University
    • Yale University
  • Udo Schwarz

    • Yale Univ
    • Yale University
  • Eric Altman

    • Center for Research on Interface Structures and Phenomena and Department of Chemical & Environmental Engineering, Yale University
    • Yale Univ
    • Yale University