Quantifying the electronic reconstruction in LaTiO$_3$/LaNiO$_3$/(LaAlO$_3$)$_3$ heterostructures using RIXS

ORAL

Abstract

A novel approach for manipulating the 3d state in transition metal oxide heterostructures has emerged with the growth of trilayer nickelate LaTiO$_3$/LaNiO$_3$/(LaAlO$_3$)$_3$ (LTNAO) (Disa et al., PRL 114 026801 (2015)). This heterostructure induces a striking reconstruction of the LaNiO$_3$ electronic structure, which is due to a combination of charge transfer from Ti's 3d state and octahedral elongation along the $c$ axis. We use resonant inelastic x-ray scattering (RIXS) experiments at Ni L$_{2,3}$ and O K edges to spectroscopically resolve the LTNAO electronic structure. Surprisingly, our results show that the octahedral elongation generates minor changes in crystal fields at Ni's 3d state compared to bulk LaNiO$_3$. Instead, heterostructuring creates an anisotropic reconstruction of the Ni 3d - O 2p hybridization. The x$^2$-y$^2$ orbital is significantly more hybridized with O p, leading to a 3z$^2$-r$^2$/x$^2$-y$^2$ hole ratio of $\sim$0.55 and large orbital polarization as measured by x-ray absorption spectroscopy. This work establishes RIXS as an ultra-sensitive probe of complex oxide heterostructures.

*Work at BNL was supported by the US Department of Energy under Award no DEAC02-98CH10886 and under Early Career Award no 20878.

Authors

  • Gilberto Fabbris

    • Brookhaven Natl Lab
    • Brookhaven National Laboratory
  • Ankit Disa

    • Yale University
    • Center for Research on Interface Structures and Phenomena and Department of Applied Physics, Yale University
  • Sohab Ismail-Beigi

    • Yale University
  • F. J. Walker

    • Yale University
    • Yale Univ
    • Center for Research on Interface Structures and Phenomena and Department of Applied Physics, Yale University
    • Center for Research on Interface Structures and Phenomena (CRISP), Yale University
  • C. H. Ahn

    • Yale University
    • Yale Univ
    • Center for Research on Interface Structures and Phenomena and Department of Applied Physics, Yale University
    • Center for Research on Interface Structures and Phenomena (CRISP), Yale University
  • Jonathan Pelliciari

    • Swiss Light Source, PSI
  • Yaobo Huang

    • Swiss Light Source, PSI
  • Thorsten Schmitt

    • Swiss Light Source, PSI
    • Swiss Light Source, Paul Scherrer Institut, Villigen, Switzerland
    • SLS PSI Villigen Switzerland
    • Paul Scherrer Institute, Switzerland
  • Lei Xu

    • IFW Dresden
  • Liviu Hozoi

    • IFW Dresden
    • IFW Dresden, Germany
    • Institute for Theoretical Solid State Physics, IFW Dresden, Germany
  • Jeroen van den Brink

    • IFW Dresden
    • Institute for Theoretical Solid State Physics, IFW Dresden
    • Institute for Theoretical Solid State Physics, IFW Dresden, Germany
    • Leibniz Institute for Solid State and Materials Research Dresden, Germany
  • Mark P. M. Dean

    • Brookhaven National Laboratory
    • Brookhaven Natl Lab