Understanding charge transport in organometal halide field effect transistors.

ORAL

Abstract

Organometal halide based perovskite are emerging materials for wide range of electronic applications. A range of optoelectronic applications like high efficiency solar cells, color pure LEDs and optical pumped lasers have been demonstrated. Here, we report the demonstration of a high performance field effect transistor fabricated from iodide perovskite material at room temperature. The devices exhibit clean saturation behavior with electron $\mu_{\mathrm{FET\thinspace }}$\textgreater 3 cm$^{\mathrm{2}}$V$^{\mathrm{-1}}$s$^{\mathrm{-1}}$ and current modulation in the range of 10$^{\mathrm{6}}$ -- 10$^{\mathrm{7}}$ which are till date the best performance achieved with these class of materials. This high performance is attributed to a combination of novel film fabrication technique and device engineering strategies. Detailed understanding of the observed band-like transport phenomenon is developed by tuning the different sources of dynamic and static disorder prevalent in the system. These finding are expected to pave way for developing next generation electronic application from perovskite materials.

*Authors acknowledge EPSRC for funding and SPS acknowledges Royal Society Newton Fellowship

Authors

  • Satyaprasad P Senanayak

    • Optoelectronics Group, Cavendish Laboratory, University of Cambridge
  • Bingyan Yang

    • Optoelectronics Group, Cavendish Laboratory, University of Cambridge
  • Aditya Sadhanala

    • Optoelectronics Group, Cavendish Laboratory, University of Cambridge
  • Prof. Sir Richard Friend

    • Optoelectronics Group, Cavendish Laboratory, University of Cambridge
  • Prof. Henning Sirrnighaus

    • Optoelectronics Group, Cavendish Laboratory, University of Cambridge