Spin-valley locking of the bulk transition-metal dichalocogenide superconductor NbSe$_{2}$

ORAL

Abstract

2H-NbSe$_{2}$ is a metallic transition metal dichalcogenide, which hosts instabilities to a charge density wave phase, and a superconducting phase at low temperatures [1]. To date, it has been assumed that these phases are largely unaffected by the spin degree of freedom. In contrast, from spin- and angle-resolved photoemission measurements, supported by first principles calculations, we reveal that the normal state Fermi surface hosts a complex spin texture. We uncover a rich spin-valley locking of the form also observed in the semiconducting materials of the same family [2], consistent with the recent observation of Ising pairing in the superconducting state of monolayer NbSe$_{2}$ [3]. We find that in the normal state of the bulk compound there is persistent spin polarisation which becomes intrinsically linked to the electronic dimensionality, showing a significant dependence on the out-of-plane momentum. This prompts a reinterpretation of the complex phases that emerge in this, and related materials. [1] Wilson JA et al, Phys. Rev. Lett. 32, 882 (1974). [2] Xiao D et al, Phys. Rev. Lett. 108, 196802 (2012); Xu X et al, Nature Phys. 10, 343–350 (2014); Riley JM et al, Nature Phys. 10, 835 (2014). [3] Xi X et al, arXiv:1507.08731.

Authors

  • L. Bawden

    • Univ of St Andrews
    • University of St Andrews
  • S. Cooil

    • Norwegian Univ of Science & Tech.
  • F. Mazzola

    • Norwegian Univ of Science & Tech.
  • J.M. Riley

    • Univ of St Andrews & Diamond Light Source
    • Univ of St Andrews and Diamond Light Source
    • University of St Andrews
  • L. Collins-McIntyre

    • Univ of St Andrews
  • Veronika Sunko

    • Univ of St Andrews & Max Planck Inst. for Chemical Physics of Solids
    • University of St Andrews
  • J. Wells

    • Norwegian Univ of Science & Tech.
  • G. Balakrishnan

    • Univ of Warwick
  • S. Bahramy

    • Univ of Tokyo & RIKEN
  • P.D.C. King

    • Univ of St Andrews
    • University of St Andrews