High-Resolution Measurements of the Roton Lifetime in Nano-Confinement

ORAL

Abstract

At very low temperatures, the phonon-roton spectrum of bulk superfluid helium is sharp and well-defined in energy. As the temperature is increased, the roton energy gap becomes smaller and the roton peak acquires a finite linewidth. The conventional understanding of this effect is that roton-roton scattering drives the softening and broadening of the roton mode where the mean free path is governed by the thermal population of rotons. It is an open question whether the roton mode follows the same behavior when the liquid is confined within sufficiently small mesopores. It is possible that the restricted geometry introduces a new length scale which controls the roton mean free path at low temperatures. We report high-resolution (~4 $\mu$eV) measurements of the roton energy and linewidth within tubular, silica nanopores 2.8 nm in diameter. The new results provide a critical test of the idea that tight, nanoscale confinement modifies the energy and linewidth of the roton excitation.

*This research was supported by NSF award DGE-1069091 and the experiment at ORNL’s Spallation Neutron Source was sponsored by the U.S. Department of Energy.

Authors

  • Matthew Bryan

    • Indiana University - Bloomington
    • Indiana Univ - Bloomington
  • Timothy Prisk

    • Oak Ridge National Lab
  • Souleymane Diallo

    • Oak Ridge National Laboratory Oak Ridge, TN, USA
    • Oak Ridge National Laboratory
    • Oak Ridge National Lab
  • Eugene Mamontov

    • Oak Ridge National Laboratory, Oak Ridge, TN, USA
    • Oak Ridge National Lab
  • Paul Sokol

    • Indiana Univ - Bloomington
    • Indiana University - Bloomington