Time Resolved X-ray Magnetic Circular Dichroism at the Linac Coherent Light Source

ORAL

Abstract

We demonstrate ultrafast time resolved X-ray Magnetic Circular Dichroism on optically switchable GdFeCo thin film samples. This method extends the element specificity of time resolved x-ray absorption spectroscopy to characterize the evolution of electron spin and orbital angular momenta. These measurements were enabled by a recent upgrade at the Linac Coherent Light Source (LCLS) to generate circularly polarized x-rays. Additionally these measurements were enhanced by new detection systems that benefit all x-ray absorption spectroscopy experiments performed in transmission. Consequently static XMCD data are in excellent agreement with similar measurements at synchrotron light sources. The LCLS is an x-ray free electron laser user facility accessible via a peer-reviewed proposal process.

*Acknowledgement: The Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515.

Authors

  • W. Schlotter

    • SLAC - Linac Coherent Light Source
    • SLAC - Natl Accelerator Lab
  • D. Higley

    • SLAC - Natl Accelerator Lab
  • E. Jal

    • SLAC - Natl Accelerator Lab
  • G. Dakovski

    • SLAC - Natl Accelerator Lab
  • E. Yuan

    • SLAC - Natl Accelerator Lab
  • J. MacArthur

    • SLAC - Natl Accelerator Lab
  • A. Lutman

    • SLAC - Natl Accelerator Lab
  • K. Hirsch

    • SLAC - Natl Accelerator Lab
  • P. Granitzka

    • SLAC - Natl Accelerator Lab
  • Z. Chen

    • SLAC - Natl Accelerator Lab
  • G. Coslovich

    • SLAC - Natl Accelerator Lab
  • M. Hoffman

    • SLAC - Natl Accelerator Lab
  • A. Mitra

    • SLAC - Natl Accelerator Lab
  • A. Reid

    • SLAC - Natl Accelerator Lab
  • P. Hart

    • SLAC - Natl Accelerator Lab
  • H.-D. Nuhn

    • SLAC - Natl Accelerator Lab
  • H. Duerr

    • SLAC - Natl Accelerator Lab
  • E. Arenholz

    • Lawrence Berkeley Natl Lab
  • P. Shafer

    • Lawrence Berkeley Natl Lab
  • P. Dennes

    • Lawrence Berkeley Natl Lab
  • J. Joseph

    • Lawrence Berkeley Natl Lab
  • L. Guyader

    • Helmholtz-Zentrum Berlin, Germany
  • A. Tsukamoto

    • Nihon University, Chiba, Japan