Antiferromagnetic order in the pyrochlores R$_{2}$Ge$_{2}$O$_{7}$ (R = Er, Yb)

ORAL

Abstract

Elastic neutron scattering, ac susceptibility, and specific heat experiments on the pyrochlores Er$_{2}$Ge$_{2}$O$_{7}$ and Yb$_{2}$Ge$_{2}$O$_{7}$ show that both systems are antiferromagnetically ordered in the $\Gamma_5$ manifold. The ground state is a $\psi_{3}$ phase for the Er sample and a $\psi_{2}$ or $\psi_{3}$ phase for the Yb sample, which suggests ``Order by Disorder"(ObD) physics. Furthermore, we unify the various magnetic ground states of all known R$_{2}$X$_{2}$O$_{7}$ (R = Er, Yb, X = Sn, Ti, Ge) compounds through the enlarged XY type exchange interaction $J_{\pm}$ under chemical pressure. The mechanism for this evolution is discussed in terms of the phase diagram proposed in the theoretical study [Wong et al., Phys. Rev. B 88, 144402, (2013)].

Authors

  • Zhiling Dun

    • University of Tennessee
    • Univ. of Tennessee, Knoxville
  • Xiang Li

    • Beijing National Laboratory for Condensed Matter Physics
  • Rafael Freitas

    • Instituto de Fisica, Universidade de Sao Paulo, Brazil
  • Everton Arrighi

    • Instituto de Fisica, Universidade de Sao Paulo, Brazil
  • Clarina Cruz

    • Oak Ridge National Laboratory
  • Minseong Lee

    • Florida State University and NHMFL
  • Eun Sang Choi

    • Florida State University and NHMFL
  • Huibo Cao

    • Oak Ridge National Laboratory
  • Harlyn Silverstein

    • University of Manitoba
  • Chris Wiebe

    • Florida State University and NHMFL, University of Manitoba, University of Winnipeg, Canadian Institute for Advanced Research
  • Jinguang Chen

    • Beijing National Laboratory for Condensed Matter Physics
  • Haidong Zhou

    • Univ. of Tennessee and NHMFL