Ambient Pressure Structural Quantum Critical Point in the Phase Diagram of (Ca$_x$Sr$_{1-x}$)$_3$Rh$_4$Sn$_{13}$
ORAL
Abstract
The quasiskutterudite superconductor Sr$_3$Rh$_4$Sn$_{13}$ features a pronounced anomaly in electrical resistivity at $T^*\sim$ 138 K. The anomaly is caused by a second-order structural transition, which can be tuned to 0 K by applying physical pressure and chemical pressure via the substitution of Ca for Sr. A broad superconducting dome is centered around the structural quantum critical point. Detailed analysis of the tuning parameter dependence of $T^*$ as well as insights from lattice dynamics calculations strongly support the existence of a structural quantum critical point at ambient pressure when the fraction of Ca is 0.9 ($x_c$=0.9). This establishes the (Ca$_x$Sr$_{1-x}$)$_3$Rh$_4$Sn$_{13}$ series as an important system for exploring the physics of structural quantum criticality and its interplay with the superconductivity, without the need of applying high pressures. Refs: Swee K. Goh {\it et al.}, Phys. Rev. Lett. {\bf 114}, 097002 (2015); Wing Chi Yu {\it et al.}, Phys. Rev. Lett. (in press, 2015)
*This work was supported by CUHK (Startup Grant, Direct Grant No. 4053071), UGC Hong Kong (ECS/24300214), Trinity College (Cam- bridge), Grants-in-Aid from MEXT (No. 22350029 and 23550152) and Glasstone Bequest (Oxford).
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