Band dependent magneto thermoelectric measurements on Ca$_3$Ru$_2$O$_7$

ORAL

Abstract

Ca$_3$Ru$_2$O$_7$ features a Neel transition at 56 K followed by a structure and metal-insulator transition at 48 K as the temperature is lowered, suggesting a complex structure-property relationship driven by electron correlated effects. However, the electronic states of Ca$_3$Ru$_2$O$_7$ are not understood. ARPES measurements revealed the presence of an electron Fermi arc, while the expected hole Fermi arc is missing. Quantum oscillations showed the existence of a small Fermi surface, but the details of the Fermi surface, including whether the hole Fermi arc is present, are not determined. We performed band-dependent thermoelectric measurement with the temperature gradient directed to a specific crystalline axis. Magneto thermopower along crystalline a and b axes, S$_a$ and S$_b$, both of which are negative in sign and nearly identical at high temperatures, were found to behave markedly differently below the metal-insulator transition, with S$_b$ changing its sign from being negative to positive. Our analysis suggests that S$_a$ and S$_b$ in Ca$_3$Ru$_2$O$_7$ are dominated by the electron and hole Fermi arcs, respectively. The implications of our data on the physics of Ca$_3$Ru$_2$O$_7$ will be discussed.

Authors

  • Hui Xing

    • Shanghai Jiao Tong Univ
    • Shanghai Jiao Tong University
  • Chenyi Shen

    • Zhejiang University
  • Libin Wen

    • Shanghai Jiao Tong University
  • Jiaming He

    • Shanghai Jiao Tong University
  • Shun Wang

    • Shanghai Jiao Tong University
  • Jin Peng

    • Tulane University
  • Jianjian Ge

    • Tulane University
  • Youming Zou

    • High Magnetic Field Laboratory, Chinese Academy of Sciences
  • Mingliang Tian

    • High Magnetic Field Laboratory, Chinese Academy of Sciences
  • Zhuan Xu

    • Zhejiang University
  • Zhiqiang Mao

    • Tulane University
  • Ying Liu

    • Pennsylvania State University, Shanghai Jiao Tong University