Isotropic and anisotropic regimes of the spin-dynamics in Sr$_{2}$IrO$_{4}$ : Field-dependent Raman scattering study

ORAL

Abstract

Experimental studies of the strong spin-orbit coupled material, Sr$_{2}$IrO$_{4}$, have provided evidence that the spin dynamics of this material can be described by an isotropic two-dimensional effective Heisenberg description. To study how well this description describes the spin-dynamics of Sr$_{2}$IrO$_{4}$ in different magnetic field regimes, in this talk, we present field-dependent Raman scattering studies of the low-energy spin-dynamics in Sr$_{2}$IrO$_{4}$. We find that for H\textgreater 1.5 T, the spin-dynamics of Sr$_{2}$IrO$_{4}$ are well described by an isotropic, 2D description. However, at low fields, H\textless 1.5 T, the spin dynamics show evidence for the effects of in-plane anisotropy and interlayer coupling. These effects must therefore be considered when modeling the low-field magnetic and dynamical properties of Sr$_{2}$IrO$_{4}$.

*This work was supported by the National Science Foundation under Grant # NSF DMR 14-64090.

Authors

  • Y. Gim

    • Physics Illinois \& Seitz MRL, University of Illinois, Urbana, IL
    • Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign, 104 South Goodwin Avenue, Urbana, Illinois 61801-2902
  • A. Sethi

    • Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign, 104 South Goodwin Avenue, Urbana, Illinois 61801-2902
  • Q. Zhao

    • Material Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA
  • J.F. Mitchell

    • Material Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA
  • G. Cao

    • Center for Advanced Materials, University of Kentucky, Lexington, Kentucky 40506, USA
  • S.L. Cooper

    • Frederick Seitz Materials Research Laboratory, University of Illinois at Urbana-Champaign, 104 South Goodwin Avenue, Urbana, Illinois 61801-2902