The role of spin fluctuations in the conductivity of CrO$_{2}$

ORAL

Abstract

Chromium dioxide is a half-metallic ferromagnet with T$_{\mathrm{C}}=$390K. Below T$_{\mathrm{C}}$, the conductivity of CrO$_{2}$ grows by two orders of magnitude and is temperature independent below about 30 K. It is believed that electron scattering by spin fluctuations is responsible for the strong temperature dependence of the conductivity. We performed time-resolved THz spectroscopy (TRTS) and time-resolved magneto-optical Kerr effect (TRMOKE) to study the role of spin fluctuations in electron conduction. A thin film CrO$_{2}$ sample was excited by an optical pump pulse. The induced conductivity changes were measured by TRTS and the induced spin response by TRMOKE. A fast and a slow component were observed in both responses. The fast component dominates the TRTS response, while the slow dominates the TRMOKE which we attribute to the spin demagnetization in CrO$_{2}$. Since the slow component contributes only a small fraction of the total conductivity change in TRTS, we conclude that spin fluctuations may not play the dominant role in the pump-induced conductivity change. We also observed that the film transmits less THz light after the pump excitation, which corresponds to it becoming more conductive. We will discuss the relationship of our observations to the electronic and optical properties of CrO$_{2}$.

*The work at Tulane was supported by the Louisiana Board of Regents through the Board of Regents Support Fund contract number LEQSF(2012-15)-RD-A-23.

Authors

  • Kate Heffernan

    • Tulane University
  • D. Talbayev

    • Tulane University
  • Xueyu Zhang

    • University of Alabama
  • A. Gupta

    • University of Alabama