Temperature dependent thermal conductivity of single- and bi- layer MoS$_{2}$ and MoSe$_{2}$

POSTER

Abstract

Thin layer transition metal dichalcogenide (TMDC) materials have received extensive interests in recent years. In this work, for the first time we systematically investigated and compared the thermal transport properties of two TMDC materials, MoS$_{2}$ and MoSe$_{2}$, and in single-layer (1L) and bi-layer (2L) forms. The optothermal Raman technique is used in the measurement process. With an improved and more robust experimental data analysis process, we discovered the thermal contact resistance and the interfacial thermal conductance of the four materials for the first time. These factors provide boundary conditions and are crucial in generating the final thermal conductivity for the suspended materials. For 1L MoS$_{2}$ and MoSe$_{2}$, the room-temperature thermal conductivities are (80 $\pm$ 17) W/mK and (72 $\pm$ 19) W/mK, respectively. For 2L MoS$_{2}$ and MoSe$_{2}$, we obtain values of (73 $\pm$ 25) and (39 $\pm$ 13)W/mK. The thermal conductivity of suspended 1L MoS$_{2}$ decreases to (66 $\pm$ 16) W/mK upon heating to 500K.

Authors

  • Xian Zhang

    • Columbia University
  • Dezheng Sun

    • Columbia University
    • Departments of Physics and Electrical Engineering, Columbia University
  • Yilei Li

    • Columbia University
    • Columbia Univ
  • Gwan-Hyoung Lee

    • Yonsei University
  • Yumeng You

    • Columbia University
  • Tony Heinz

    • Columbia University
  • James Hone

    • Columbia University
  • Xu Cui

    • Columbia University