Disorder induced correlation gap suppresses superconductivity in the 5$d$ metallic perovskite Ba$_{1-x}$La$_{x}$PbO$_{3}$

POSTER

Abstract

We report the synthesis and characterization of the electronic structure of thin films of the perovskite Ba$_{1-x}$La$_{x}$PbO$_{3}$ grown by oxide molecular-beam epitaxy. Using angle-resolved photoemission spectroscopy our measurements reveal a Fermi surface consistent with density functional calculations at low doping, but indicate the formation of an energy gap at higher doping values ($x$ $\sim$ 0.2), consistent with electrical transport measurements. By comparison with temperature-dependent point contact tunneling spectroscopy measurements, we show this behavior is consistent with a disorder-driven correlation gap. Moreover the photoemission data reveal a density of states that is not linear at high binding energies, suggesting discrepancy with previous tunneling density of states measurements of superconducting oxides.

Authors

  • Carolina Adamo

    • Stanford University
  • Daniel Shai

    • Cornell University
  • Bredan Faeth

    • Cornell University
  • Philip Wu

    • Stanford University
  • Kyle Shen

    • Cornell University
  • Darrell Schlom

    • Cornell University
  • Malcolm Beasley

    • Stanford University