Crystal structure and physical properties of Cr oxide with K$_{2}$NiF$_{4}$-type structure

POSTER

Abstract

Ruddlesden-Popper (RP) type structure materials have been attracted much attention due to their interesting physical properties including high-$T_{\mathrm{c}}$ superconductivity, charge stripe, itinerant ferromagnetism and so on. In this work we are presenting physical properties of some of the K$_{2}$NiF$_{4}$ type structure compounds. YSrCrO$_{4}$ is first synthesized and found to be a hetto-type K$_{2}$NiF$_{4}$ structure. The space group of YSrCrO$_{4}$ is determined to be orthorhombic Pccn by the electron diffraction and the powder X-ray diffraction. YSrCrO$_{4}$ shows two-dimensional (2D) spin correlations and a canted antiferromagnetic (AF) ordering. Evidence of AF ordering of the Cr oxides is obtained microscopically from ESR. The dielectric measurements suggest existence of in-gap states, while no magneto-dielectric coupling was observed in the above compounds.

Authors

  • Ting-Hui Kao

    • National Sun-Yet Sen University, Kaohsiung 804, Taiwan
  • Hiroya Sakurai

    • National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
  • Taras Kolodiazhnyi

    • National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan
  • Yutaro Suzuki

    • Nagoya Institute of Technology, Nagoya 466-855, Japan
  • Momoko Okabe

    • Nagoya Institute of Technology, Nagoya 466-855, Japan
  • Toru Asaka

    • Nagoya Institute of Technology, Nagoya 466-855, Japan
  • Koichiro Fukuda

    • Nagoya Institute of Technology, Nagoya 466-855, Japan
  • Susumu Okubo

    • Kobe University, 1-1 Rokkodai-cho, Nada, Kobe 657-8501, Japan
  • Shohei Ikeda

    • Kobe University, 1-1 Rokkodai-cho, Nada, Kobe 657-8501, Japan
  • Shigeo Hara

    • Kobe University, 1-1 Rokkodai-cho, Nada, Kobe 657-8501, Japan
  • Takahiro Sakurai

    • Kobe University, 1-1 Rokkodai-cho, Nada, Kobe 657-8501, Japan
  • Hitoshi Ohta

    • Kobe University, 1-1 Rokkodai-cho, Nada, Kobe 657-8501, Japan
  • Hung-Duen Yang

    • National Sun-Yet Sen University, Kaohsiung 804, Taiwan
    • Department of Physics, National Sun Yat Sen University, Taiwan
    • Natl Sun Yat Sen Univ