Spin-orbital fluctuations in the paramagnetic Mott insulator (V$_{1-x}$Cr$_x$)$_2$O$_3$

ORAL

Abstract

The phase diagram of rhombohedral V$_2$O$_3$ features several distinct strongly correlated phases as a function of doping, pressure and temperature. When doped with chromium for 180 K$<$T$<$450 K the material undergoes a Mott metal to insulator transition. Using the modern time-of-flight neutron scattering spectrometer SEQUOIA at the SNS, we have probed the excitation spectrum of (V$_{0.96}$Cr$_{0.04}$)$_2$O$_3$ in the PI phase and in the monoclinic commensurate anti-ferromagnet for T$<$180 K. An effective exchange Hamiltonian that accounts for the low T spin waves indicates alternating FM and AFM interactions for nearest neighbor spin pairs that are equivalent in the PI. We argue that the corresponding spin-orbital fluctuations are responsible for the extremely short-range dynamic spin correlations that we document in the PI phase.

*Research at the Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Research was also supported by ORNL LDRD funding.

Authors

  • Jonathan Leiner

    • Oak Ridge National Lab
  • Matthew Stone

    • Oak Ridge National Lab
  • Mark Lumsden

    • Oak Ridge National Lab
  • Wei Bao

    • Renmin University of China
  • Collin Broholm

    • Johns Hopkins University