Magnetism and magnetic ordering in \textit{Ln}CuGa$_{3}$ (\textit{Ln} $=$ lanthanide)
ORAL
Abstract
We report structural characterization and magnetization and transport measurements on \textit{Ln}CuGa$_{3}$ (\textit{Ln} $=$ La, Ce, Pr, Nd, Sm, Eu, and Gd) intermetallics. Magnetization in fixed field was measured for high quality polycrystalline samples at temperatures between 1.8 and 300 K, along with the isothermal variation of magnetization with field, while the temperature dependent resistivity was measured down to $T = $ 0.3 K. All members of this family, except for the PrCuGa$_{3}$ and non-magnetic LaCuGa$_{3}$ compounds, exhibit magnetic ordering above 1.8 K at temperatures ranging from 2 K (CeCuGa$_{3})$ to 75 K (EuCuGa$_{3})$. The Eu and Sm based compounds exhibit multiple magnetic transitions. SmCuGa$_{3}$ appears to be ferromagnetic, whereas the other compounds order antiferromagnetically. Preliminary studies on single crystals of SmCuGa$_{3}$ indicate that the ordered moments lie parallel to the $c$-axis in the low temperature magnetically ordered phase of this tetragonal system.
*Supported in part by NSF DMR-1337567, DST Grant SR/S2/RJN-24/2010. and the CSIR
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