Evidence of magnetic clusters in the disordered ferromagnet Ni-V close to the quantum critical concentration

ORAL

Abstract

We report the results of muon spin relaxation ($\mu$SR) experiments in zero field (ZF) and transverse field (TF) as well as magnetization (M) data of Ni$_{1-x}$V$_{x}$ close to the critical vanadium concentration $x_c \approx11.6\%$ where the onset of the ferromagnetic (FM) order is suppressed. This material features a prototypical disordered quantum phase transition (QPT) as seen in the temperature (T) and magnetic field (H) dependence of $M(H,T)$. In the paramagnetic phase (PM) above $x_c$, $M(H,T)$ is well described by non-universal power laws characterized by an exponent $\alpha(x-x_c)$, establishing a quantum Griffiths phase. Here, we focus on the FM side of the QPT below $x_c$. After subtracting the spontaneous magnetization $M_0$, we find that $M(H,T)-M_0$ also follows a power law in $H$ at low $T$ with an analogous non-universal exponent $\alpha(x_c-x)$. This is the first evidence of a quantum Griffiths phase within the FM phase in this disordered alloy. $\mu$SR in ZF recognized a broad field distribution below $x_c$ as evidence of magnetic spatial inhomogeneities in the FM phase. Different muon depolarization rates in TF and ZF reveal magnetic clusters already in the PM regime. These observed clusters are important generic ingredients of a disordered QPT.

Authors

  • Ruizhe Wang

    • Kent State University, Kent, OH
  • S. Ubaid-Kassis

    • Kent State University, Kent, OH
  • A. Schroeder

    • Kent State University, Kent, OH
  • P.J. Baker

    • ISIS Facility, U.K.
  • F.L. Pratt

    • ISIS Facility, U.K.
  • S.J. Blundell

    • Univerisity of Oxford, U.K.
  • T. Lancaster

    • Univerisity of Oxford, U.K.
  • I. Franke

    • Univerisity of Oxford, U.K.
  • J.S. Moeller

    • Univerisity of Oxford, U.K.
  • T. Vojta

    • Missouri University of S \& T, Rolla, MO