Investigation of magnetic order in Sm${Tr}$$_2$Zn$_{20}$ (${Tr}$ = Fe, Co, Ru) and Sm${Tr}$$_2$Cd$_{20}$ (${Tr}$ = Ni, Pd)

ORAL

Abstract

Single crystals of the cage compounds Sm${Tr}$$_2$Zn$_{20}$ (${Tr}$ = Fe, Co, Ru) and Sm${Tr}$$_2$Cd$_{20}$ (${Tr}$ = Ni, Pd) have been investigated by means of electrical resistivity, magnetization, and specific heat measurements. The compounds SmFe$_{2}$Zn$_{20}$, SmRu$_{2}$Zn$_{20}$, and SmNi$_{2}$Cd$_{20}$ exhibit ferromagnetic order with Curie temperatures of $T_C$ = 47.4 K, 7.6 K, and 7.5 K, respectively, whereas SmPd$_{2}$Cd$_{20}$ is an antiferromagnet with a N\'{e}el temperature of $T_N$ = 3.4 K. No evidence for magnetic order is observed in SmCo$_{2}$Zn$_{20}$ down to 110 mK. The Sommerfeld coefficients $\gamma$ are found to be 57 mJ/mol-K$^2$ for SmFe$_{2}$Zn$_{20}$, 79.5 mJ/mol-K$^2$ for SmCo$_{2}$Zn$_{20}$, 258 mJ/mol-K$^2$ for SmRu$_{2}$Zn$_{20}$, 165 mJ/mol-K$^2$ for SmNi$_{2}$Cd$_{20}$, and 208 mJ/mol-K$^2$ for SmPd$_{2}$Cd$_{20}$. Enhanced values of Sommerfeld coefficients $\gamma$ and a quadratic temperature dependence of the electrical resistivity at low temperature for SmRu$_{2}$Zn$_{20}$ and SmPd$_{2}$Cd$_{20}$ suggest an enhancement of the quasiparticle masses due to hybridization between localized 4$f$ and conduction electron states.

*Research at UCSD was supported by the U. S. DOE under Grant No. DE-FG02-04-ER46105 and the U. S. NSF under Award Grant No. DMR 1206553. Research at California State University, Fresno was supported by the U. S. NSF under Grant No. DMR 1104544

Authors

  • D. Yazici

    • Physics Department, UC San Diego
    • Department of Physics, University of California, San Diego
    • UC, San Diego
    • Department of Physics, University of California, San Diego, La Jolla, CA 92093, USA
  • B. D. White

    • UC, San Diego
  • P.-C. Ho

    • California State University, Fresno
  • N. Kanchanavatee

    • UC, San Diego
  • K. Huang

    • UC, San Diego
  • N. R. Dilley

    • Quantum Design
  • M. B. Maple

    • UC, San Diego