Doping Dependence of the Structural and Magnetic Properties of CeCu$_{6-x}$T$_{x}$ (T = Ag, Pd)

ORAL

Abstract

CeCu$_{6-x}$Au$_x$ is a well-known heavy fermion system that exhibits an antiferromagnetic quantum critical point(QCP) at x $\sim$ 0.1. The end-member, CeCu$_6$ undergoes a structural transition, which is suppressed as Cu is partially substituted by Au in CeCu$_{6-x}$Au$_x$: the critical concentration being at x$\sim$0.1. This critical point occurs in close proximity to the antiferromagnetic QCP. Here, we study related systems, CeCu$_{6-x}$Ag$_x$ and CeCu$_{6-x}$Pd$_x$, to determine more globally the role of structural degrees of freedom in the observed critical behavior. For magnetically ordered compositions of CeCu$_{6-x}$Ag$_x$ and CeCu$_{6-x}$Pd$_x$, we find a long-range order with the wave-vector similar to that observed in CeCu$_{6-x}$Au$_x$. The structural transition temperature of CeCu$_{6-x}$Ag$_x$ decreases linearly with Ag concentration until the transition is completely suppressed at x$\sim$0.1. In contrast, moderate Pd-doping does not affect the structural transition, which is observed in CeCu$_{6-x}$Pd$_x$ with x $\leq$ 0.4.

Authors

  • L. Poudel

    • Univ of Tennessee, Knoxville and Oak Ridge National Laboratory
  • M.A. McGuire

    • Oak Ridge National Laboratory
  • C. de la Cruz

    • Oak Ridge National Laboratory
  • S. Calder

    • Oak Ridge National Laboratory
  • A.F. May

    • Oak Ridge National Laboratory
  • W. Tian

    • Oak Ridge National Laboratory
  • M. Matsuda

    • Oak Ridge National Laboratory
  • H.B. Cao

    • Oak Ridge National Laboratory
  • T. Hong

    • Oak Ridge National Laboratory
  • A.E. Payzant

    • Oak Ridge National Laboratory
  • H. Jeen

    • Oak Ridge National Laboratory and Pusan National University, S. Korea
  • H.N. Lee

    • Oak Ridge National Laboratory
  • M. Koehler

    • Univ. of Tennessee, Knoxville
  • H. Zhou

    • Univ. of Tennessee, Knoxville
  • V. Keppens

    • Univ. of Tennessee, Knoxville
  • D. Mandrus

    • Univ. of Tennessee, Knoxville and Oak Ridge National Laboratory
  • A.D. Christianson

    • Univ. of Tennessee, Knoxville and Oak Ridge National Laboratory