Magnetic field induced directional dichroism of spin waves in multiferroic BiFeO$_3$ at THz frequencies
ORAL
Abstract
Using far infrared spectroscopy in high magnetic fields we show that spin excitations in BiFeO$_3$ simultaneously interact with the electric and magnetic field components of light resulting in directional dichroism (DD) of absorption. DD in BiFeO$_3$ arises because an applied static magnetic field induces a toroidal moment in the cycloidal spin structure. Strong DD is observed even in the room-temperature state of the material. The results are explained on the microscopic level as an interplay of five different interactions: isotropic exchange couplings between nearest and next nearest neighbors, an easy-axis anisotropy along the ferroelectric polarization, Dzyaloshinskii-Moriya (DM) interaction that creates the cycloid and DM interaction that causes spin canting.
*Research sponsored by the Estonian Ministry of Education and Research (IUT23-3), Estonian Science Foundation (ETF8703), and U.S. Department of Energy (JL), Office of Science, Materials Sciences and Engineering Division (RF and JL) and Office of Basis En
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