Magnetic field induced directional dichroism of spin waves in multiferroic BiFeO$_3$ at THz frequencies

ORAL

Abstract

Using far infrared spectroscopy in high magnetic fields we show that spin excitations in BiFeO$_3$ simultaneously interact with the electric and magnetic field components of light resulting in directional dichroism (DD) of absorption. DD in BiFeO$_3$ arises because an applied static magnetic field induces a toroidal moment in the cycloidal spin structure. Strong DD is observed even in the room-temperature state of the material. The results are explained on the microscopic level as an interplay of five different interactions: isotropic exchange couplings between nearest and next nearest neighbors, an easy-axis anisotropy along the ferroelectric polarization, Dzyaloshinskii-Moriya (DM) interaction that creates the cycloid and DM interaction that causes spin canting.

*Research sponsored by the Estonian Ministry of Education and Research (IUT23-3), Estonian Science Foundation (ETF8703), and U.S. Department of Energy (JL), Office of Science, Materials Sciences and Engineering Division (RF and JL) and Office of Basis En

Authors

  • Urmas Nagel

    • Nat.-l Inst. of Chem. Phys. \& Biophys., Tallinn, Estonia
  • T. R\~o\~om

    • Nat.-l Inst. of Chem. Phys. \& Biophys., Tallinn, Estonia
  • S. Bord\'acs

    • Budapest University of Technology and Economics, Hungary
  • I. K\'ezsm\'arki

    • Budapest University of Technology and Economics, Hungary
  • H.T. Yi

    • Rutgers Univ., New Jersey
  • S.-W. Cheong

    • Rutgers Univ., New Jersey
  • Jun Hee Lee

    • Oak Ridge National Laboratory, Tennessee
  • Randy S. Fishman

    • Oak Ridge National Laboratory, Tennessee