Imaging Dirac-Mass Disorder from Magnetic Dopant-Atoms in the Ferromagnetic Topological Insulator Cr$_{\mathrm{x}}$(Bi$_{0.1}$Sb$_{0.9})_{\mathrm{2-x}}$Te$_{3}$ -- Part I

ORAL

Abstract

Topological insulators (TI) have a gapless surface state of Dirac fermions protected by the time reversal symmetry (TRS). However, TRS can be broken in the ferromagnetic state induced by magnetic doping. This leads to the opening of ``mass gap'' at the Dirac point. Such a gap is predicted to involve many exotic phenomena for which understanding the microscopic role of magnetic dopants is critical. But it is unknown how the spatial arrangements of the magnetic dopant atoms influence the Dirac-mass gap at the atomic scale. Here we image the locations of the magnetic (Cr) dopant atoms in the ferromagnetic TI Cr$_{0.08}$(Bi$_{0.1}$Sb$_{0.9})_{1.92}$Te$_{3}$. Simultaneous visualization of the Dirac-mass gap $\Delta $(r) reveals its intense disorder, which we demonstrate directly is related to fluctuations in n(r), the areal Cr atom density at the surface. The relationship of the surface-state Fermi wavevectors to both the correlation length and anisotropic structure of $\Delta $(r) are found consistent with predictions for ferromagnetism mediated by the surface states.

Authors

  • Chung Koo Kim

    • Brookhaven National Laboratory
    • BNL
    • CMPMS Brookhaven National Lab, Cornell University
  • Inhee Lee

    • Brookhaven National Laboratory
    • BNL
  • Jinho Lee

    • Seoul National University
    • BNL, SNU
  • Simon Billinge

    • Columbia University
    • BNL, Columbia
  • Ruidan Zhong

    • Brookhaven National Laboratory
    • Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, NY 11973, USA
    • BNL, Stony Brook
    • Brookhaven National Lab
  • John Schneeloch

    • Brookhaven National Laboratory
    • Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, NY 11973, USA
    • Brookhaven Natl Lab
    • BNL, Stony Brook
    • Brookhaven National Lab
  • Tiansheng Liu

    • BNL, N Univ of China
  • John Tranquada

    • Brookhaven National Laboratory
    • Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, NY 11973, USA
    • Brookhaven Natl Lab
    • BNl
  • Genda Gu

    • Brookhaven National Lab
    • Brookhaven National Laboratory
    • Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, NY 11973, USA
    • Brookhaven Natl Lab
    • BNL
    • Department of Physics, Brookhaven National Laboratory
    • Brookhaven National Lab, Upton, NY
    • University of Colorado at Boulder
  • J.C. Davis

    • Cornell University
    • BNL, Cornell, U of St. Andrews, Kavli Inst. at Cornell
    • Cornell University, CMPMS Brookhaven National Lab, University of St. Andrews, Kavli Institute at Cornell for Nanoscale Science