Fragile antiferromagnetism in the heavy-fermion compound YbBiPt
COFFEE_KLATCH · Invited
Abstract
The discovery of YbBiPt [1] generated strong interest due to its extraordinary Sommerfield coefficient ($\gamma \approx $ 8 J/mol-K$^{2})$ and the fact that all of its relevant energy scales including the Kondo temperature, Weiss temperature, crystal field splitting, and a proposed antiferromagnetic (AFM) ordering below $T_{\textrm{N}} =$ 0.4 K are small and comparable, suggesting a complex interplay of competing interactions at low temperature. Much of the recent attention on YbBiPt has focused on the possibility of a magnetic-field-tuned AFM quantum critical point occurring at a low critical magnetic field of $\mu_{0}H_{\textrm{c}}$ = 0.4 T [2]. Although thermodynamic and transport measurements in ambient fields suggested that YbBiPt manifests AFM order below $T_{\textrm{N}}$, scattering measurements over the past 22 years failed to identify magnetic ordering in powder or single-crystal samples. In this talk, I will present recent elastic and inelastic neutron scattering experiments on single crystals of YbBiPt that demonstrated clear scattering signatures of unusual AFM order at low temperature [3]. The ambient field elastic scattering consists of two components: a narrower component that appears below $T_{\textrm{N}} \approx $ 0.4 K, which can be identified with features observed in the bulk transport measurements; and a broad scattering component that persists up to $T^{\ast} \approx $ 0.7 K corresponding to AFM correlations extending over $\approx $ 20 {\AA}.\\[4pt] [1] P. C. Canfield \textit{et al}., J. Appl. Phys. \textbf{70}, 5800 (1991); Z. Fisk \textit{et al}., Phys. Rev. Lett. \textbf{67}, 3310 (1991).\\[0pt] [2] E. D. Mun \textit{et al}., Phys. Rev. B \textbf{87}, 075120 (2013).\\[0pt] [3] B. G. Ueland\textit{ et al}., Phys. Rev. B \textbf{89}, 180403(R) (2014).
*This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Ames Laboratory is operated for the U.S. DOE by Iowa State University under contract \# DE-AC02-07CH1135
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