Brownmillerite CaCoO$_{2.5}$: Synthesis, Re-entrant Structural Transitions and Magnetic properties

ORAL

Abstract

Cobalt oxides attract both fundamental and technological attention due to their physical properties including thermoelectricity, giant magnetoresistance, superconductivity and multiferroicity [1]. Here we report the first synthesis of CaCoO$_{2.5}$ single crystals using a high pressure optical-image floating zone technique. We find that it is an ordered oxygen-deficient perovskite of the brownmillerite type, and it undergoes an unprecedented re-entrant structural phase transitions (Pcmb$\to $ P2/c11$\to $ P12$_{1}$/m1$\to $ Pcmb) with decreasing temperature. We describe its temperature-dependent structural, thermal, and magnetic properties, including AFM ordering near 240 K, with a weakly spin canted ferromagnet ground state below 140 K. The magnetic response of CaCoO$_{2.5}$ depends markedly on the cooling rate and field history. Magnetization data also imply the potential of a distinct, field-induced phase arising uniquely from the P12$_{1}$/m1 structure, revealed as kinetically trapped by a rapid-cooling protocol.\\[4pt] [1] Raveau, B.; Seikh, M. M. Cobalt Oxides: From Crystal Chemistry to Physics; Wiley-VCH: Weinheim, 2012.

*Work in the Materials Science Division at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Division of Materials Science and Engineering.

Authors

  • Junjie Zhang

    • Argonne Natl Lab
  • Hong Zheng

    • Argonne Natl Lab
  • Christos Malliakas

    • Argonne Natl Lab
  • Jared Allred

    • Argonne National Laboratory (ANL)
    • Materials Science Division, Argonne National Laboratory
    • Argonne National Laboratory
    • Argonne Natl Lab
  • Yang Ren

    • Argonne Natl Lab
  • Qing'an Li

    • Argonne Natl Lab
  • Tianheng Han

    • Argonne Natl Lab
  • John Mitchell

    • Argonne National Laboratory
    • Argonne Natl Lab