Charge-density waves competitions in 1T-TaS$_{2}$ and ErTe$_{3}$ investigated by femtosecond electron crystallography

ORAL

Abstract

Competitions between different lattice- and charge-ordered states in two-dimensional materials can lead to strongly first order phase transitions. In 1T-TaS$_{2}$, the phase transitions are primarily driven by strong electron correlations and Fermi surface nesting, but between the Mott insulating ground state and the high-temperature incommensurate charge-density wave (CDW) there exists a near-commensurate phase characterized by unique domain structures, where their long-range coherence and pseudo-gap property are currently under debates. Using femtosecond electron crystallography, we resolved the domain proliferation dynamics and the distinctly different characters of electronic phase transitions and CDW restructuring. We also compare our results with the CDW competitions in the weakly correlated system ErTe$_{3}$.

*Our work is supported by Department of Energy under Grant No. DE-FG02-06ER46309.

Authors

  • Faran Zhou

    • Michigan State University
  • Tzong-Ru Han

    • Michigan State University
  • Zhensheng Tao

    • Michigan State University
  • Jenni Portman

    • Michigan State University
  • Dat Do

    • Michigan State University
  • Subhendra Mahanti

    • Michigan State University
  • Phillip Duxbury

    • Michigan State University
  • Chong-Yu Ruan

    • Michigan State University
  • Christos Malliakas

    • Northwestern University
  • Mercouri Kanatzidis

    • Northwestern University