Full magnetic dispersion relation in the frustrated quasi-1D ferromagnet Ca$_2$Y$_2$Cu$_5$O$_{10}$

ORAL

Abstract

Ca$_2$Y$_2$Cu$_5$O$_{10}$ consists of edge-sharing CuO$_2$ chains, in which Cu$^{2+}$ ions carry spin 1/2. The nearest-neighbor ($J_1$) and the next-nearest-neighbor interaction ($J_2$) are ferromagnetic and antiferromagnetic, respectively. For the $J_1$-$J_2$ model the theory predicts that when the ratio $\alpha$(=$|J_2/J_1|$) becomes larger than 0.25, the ground state becomes a spiral state. For the aforementioned compound, Kuzian et al. determined $\alpha$ to be 0.19, which is close to the critical value [1]. However, the parameters were fitted using the observed data up to $\sim$10 meV, above which the magnetic excitations were found to be broadened [2]. In order to determine the overall dispersion relation, we performed inelastic neutron scattering experiments using the HYSPEC neutron spectrometer at the SNS. We succeeded in observing the full magnetic dispersion that extends up to $\sim$55 meV. As previously observed, the magnetic excitations appeared to almost vanish at $\sim$11.5 meV. We also found another noticeable gap-like behavior at $\sim$28 meV. We re-evaluate the essential exchange coupling parameters and discuss the origin of gap-like regions in the spin-wave dispersion. [1] R. O. Kuzian et al., PRL109, 117207 (2012). [2] M. Matsuda et al., PRB63, 180403 (2001).

Authors

  • Masaaki Matsuda

    • Quantum Condensed Matter Division, Oak Ridge National Laboratory
    • Oak RIdge Natl Lab
    • Oak Ridge National Lab
  • J. Ma

    • Quantum Condensed Matter Division, Oak Ridge National Laboratory
  • V. O. Garlea

    • Quantum Condensed Matter Division, Oak Ridge National Laboratory
  • S. Nishimoto

    • Inst. for Theoretical Solid State Physics, IFW Dresden, Germany
  • S.-L. Drechsler

    • Inst. for Theoretical Solid State Physics, IFW Dresden, Germany
  • R. O. Kuzian

    • Inst. f. Problems of Materials Science NASU, Kyiv, Ukraine
  • T. Ito

    • National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Japan
  • H. Yamaguchi

    • National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Japan
  • K. Oka

    • National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Japan