Nano-architectures of flattened polymer chains at solid-polymer melt interface

POSTER

Abstract

Our group has recently revealed that, by using x-ray/neutron reflectivity, irreversibly adsorbed polystyrene (PS) layers onto planar silicon substrates are composed of the two different nano-architectures: flattened chains that constitute the inner higher density region of the adsorbed layers and loosely adsorbed polymer chains that form the outer bulk-like density region. Here, we focus on the following two effects on the formation of the flattened layer: (i) intramolecular architectures and (ii) polymer/substrate interactions. Various surface sensitive techniques including in-situ x-ray/neutron reflectivity, grazing incidence X-ray diffraction, and atomic force microscope were utilized to illuminate the inherent chain architectures at the solid/polymer interface.

*Acknowledgement: We acknowledge the financial support from NSF Grant No. CMMI-084626.

Authors

  • Xiaoyu Di

    • Department of Materials Science and Engineering, Stony Brook University, Stony Brook, NY 11794-2275
  • Jiaxun Wang

    • Department of Materials Science and Engineering, Stony Brook University, Stony Brook, NY 11794-2275
  • Naisheng Jiang

    • Department of Materials Science and Engineering, Stony Brook University, Stony Brook, NY 11794-2275
  • Maya K. Endoh

    • Department of Materials Science and Engineering, Stony Brook University, Stony Brook, NY 11794-2275
  • Tadanori Koga

    • Department of Materials Science and Engineering, Stony Brook University, Stony Brook, NY 11794-2275
  • Masafumi Fukuto

    • Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, NY 11973, USA
  • Takamichi Shinohara

    • Institute for Materials Chemistry and Engineering, Kyushu University, Motooka, Nishi-ku, Fukuoka 819-0395, Japan
  • Atsushi Takahara

    • Institute for Materials Chemistry and Engineering, Kyushu University, Motooka, Nishi-ku, Fukuoka 819-0395, Japan