Valence band study of Sm$_{0.1}$Ca$_{0.9-x}$Sr$_{\mathrm{x}}$MnO$_{3}$ using high resolution photoemission spectroscopy

ORAL

Abstract

We have studied the valence band electronic structure of Sm$_{0.1}$Ca$_{\mathrm{0.9-x}}$Sr$_{\mathrm{x}}$MnO$_{3}$ (x $=$ 0, 0.1, 0.3 and 0.6) at various temperatures using high resolution photoemission spectroscopy (HRPES). The data were taken using a Scienta R4000 energy analyser and the resolution was set at 5 meV. The doping dependent studies of Sm$_{0.1}$Ca$_{\mathrm{0.9-x}}$Sr$_{\mathrm{x}}$MnO$_{3}$ at 50 K, 100 K and 295 K are quite interesting. The density of e$_{\mathrm{g}}$ states near the Fermi level decreases with Sr substitution at the Ca site at 50 K. Also the similar trend has been observed at 100 K. At 295 K the changes in the e$_{\mathrm{g}}$ states is quite different than the earlier temperatures where the intensity remains the same for x $=$ 0, 0.1 and 0.3 and then decreases for x $=$ 0.6. These changes in the density of states near the Fermi level will be explained by taking into account the structural, electrical and magnetic properties associated with this system.

*Permanent affiliation of Manas Kumar Dalai ; CSIR-National Physical Laboratory, New Delhi-110012, India. MKD acknowledges the Indo-US Science and Technology Forum (IUSSTF) for the fellowship.

Authors

  • Manas Kumar Dalai

    • Department of Physics, University of Illinois at Urbana Champaign, 1110 West Green Street, Urbana, IL 61801, USA
  • Biju Raja Sekhar

    • Institute of Physics, Sachivalaya Marg, Bhubaneswar - 751005, India
  • Deepnarayan Biswas

    • Department of Condensed Matter Physics and Materials' Science, Tata Institute of Fundamental Research, Colaba, Mumbai 400 005, India
  • Sangeeta Thakur

    • Department of Condensed Matter Physics and Materials' Science, Tata Institute of Fundamental Research, Colaba, Mumbai 400 005, India
  • Kalobaran Maiti

    • Department of Condensed Matter Physics and Materials' Science, Tata Institute of Fundamental Research, Colaba, Mumbai 400 005, India
  • Tai-Chang Chiang

    • Department of Physics, University of Illinois at Urbana Champaign, 1110 West Green Street, Urbana, IL 61801, USA
  • Christine Martin

    • Laboratoire CRISMAT, CNRS UMR 6508, 6 Boulevard Mar\'echal Juin, 14050 Caen cedex, France