Doping influence of spin dynamics and magnetoelectric effect in hexagonal Y$_{0.7}$Lu$_{0.3}$MnO$_3$

ORAL

Abstract

Inelastic neutron scattering experiments were performed to study spin waves and their correlation with the magnetoelectric effect in Y$_{0.7}$Lu$_{0.3}$MnO$_3$. The Mn trimerization distortion has been suggested to play a key role in determining the magnetic structure and the magnetoelectric effect in YMnO$_3$ and LuMnO$_3$. In Y$_{0.7}$Lu$_{0.3}$MnO$_3$, our INS study reveals a much smaller in-plane (hexagonal \textit{ab}-plane) anisotropy gap that coincides with a weaker in-plane dielectric anomaly at $T_N$. Since both the smaller in-plane anisotropy gap and the weaker in-plane dielectric anomaly are coupled to a weaker Mn trimerization distortion in Y$_{0.7}$Lu$_{0.3}$MnO$_3$ comparing to YMnO$_3$ and LuMnO$_3$, we conclude that the Mn trimerization is responsible for the magnetoelectric effect and multiferroic phenomenon in Y$_{1-x}$LuxMnO$_3$.

Authors

  • Wei Tian

    • Oak Ridge National Laboratory
  • Guotai Tan

    • University of Tennessee and Beijing Normal University
  • Liu Liu

    • Beijing Normal University
  • Jinxing Zhang

    • Beijing Normal University
  • Barry Winn

    • Oak Ridge National Laboratory
  • Tao Hong

    • Oak Ridge National Laboratory
  • Jaime Fernandez-Baca

    • Oak Ridge National Laboratory
  • Chenglin Zhang

    • University of Tennessee and Rice University
  • Pengcheng Dai

    • University of Tennessee and Rice University